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Tunable nanowire nonlinear optical probe

机译:可调谐纳米线非线性光学探头

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One crucial challenge for subwavelength optics has been the development of a tunable source of coherent laser radiation for use in the physical, information and biological sciences that is stable at room temperature and physiological conditions. Current advanced near-field imaging techniques using fibre-optic scattering probes have already achieved spatial resolution down to the 20-nm range. Recently reported far-field approaches for optical microscopy, including stimulated emission depletion, structured illumination, and photoactivated localization microscopy, have enabled impressive, theoretically unlimited spatial resolution of fluorescent bio-molecular complexes. Previous work with laser tweezers has suggested that optical traps could be used to create novel spatial probes and sensors. Inorganic nanowires have diameters substantially below the wavelength of visible light and have electronic and optical properties that make them ideal for subwavelength laser and imaging technology. Here we report the development of an electrode-free, continuously tunable coherent visible light source compatible with physiological environments, from individual potassium niobate (KNbO_3) nanowires. These wires exhibit efficient second harmonic generation, and act as frequency converters, allowing the local synthesis of a wide range of colours via sum and difference frequency generation. We use this tunable nanometric light source to implement a novel form of subwavelength microscopy, in which an infrared laser is used to optically trap and scan a nanowire over a sample, suggesting a wide range of potential applications in physics, chemistry, materials science and biology.
机译:亚波长光学器件的一项关键挑战是开发一种可调谐的相干激光辐射源,用于物理,信息和生物科学,该光源在室温和生理条件下稳定。当前使用光纤散射探针的先进近场成像技术已经实现了低至20 nm范围的空间分辨率。最近报道的光学显微镜远场方法,包括受激发射损耗,结构化照明和光活化定位显微镜,已使荧光生物分子复合物具有令人印象深刻的,理论上无限的空间分辨率。以前使用激光镊子进行的工作表明,可以使用光阱来创建新颖的空间探头和传感器。无机纳米线的直径大大低于可见光的波长,并且具有电子和光学特性,使其非常适合亚波长激光和成像技术。在这里,我们从单个铌酸钾(KNbO_3)纳米线报告了与生理环境兼容的无电极,连续可调的相干可见光源的开发。这些导线表现出有效的二次谐波生成,并充当变频器,从而允许通过和频和差频生成来对各种颜色进行本地合成。我们使用这种可调纳米光源来实现一种新型的亚波长显微镜,其中使用红外激光光学捕获并扫描样品上的纳米线,这表明在物理,化学,材料科学和生物学中的广泛应用潜力。

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