Selective catalytic reduction converter design: The effect of ammonia nonuniformity at inlet

摘要

A three-dimensional CFD model of SCR converter with detailed chemistry is developed. The model is used to study the effects of radial variation in inlet ammonia profile on SCR emission performance at different temperatures. The model shows that radial variation in inlet ammonia concentration affects the SCR performance in the operating range of 200-400 ℃. In automotive SCR systems, ammonia is non-uniformly distributed due to evaporation/reaction of injected urea, and using a ID model or a 3D model with flat ammonia profile at inlet for these conditions can result in erroneous emission prediction. The 3D SCR model is also used to study the effect of converter design parameters like inlet cone angle and monolith cell density on the SCR performance for a non-uniform ammonia concentration profile at the inlet. The performance of SCR is evaluated using DeNO, efficiency and ammonia slip.