Ni-Catalyzed Site-Selective Dicarboxylation of 1,3-Dienes with CO_2

Andreu Tortajada; Ryo Ninokata; Ruben Martin

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Ni-Catalyzed Site-Selective Dicarboxylation of 1,3-Dienes with CO_2

机译：Ni催化CO_2催化1,3-二烯的位点选择性二羧基化

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摘要

A site-selective catalytic incorporation of multiple CO_(2) molecules into 1,3-dienes en route to adipic acids is described. This protocol is characterized by its mild conditions, excellent chemo- and regioselectivity and ease of execution under CO_(2) (1 atm), including the use of bulk butadiene and/or isoprene feedstocks.

机译：描述了在向己二酸的途中将多个CO_（2）分子选择性地掺入1,3-二烯的过程。该协议的特点是条件温和，出色的化学和区域选择性以及在CO_（2）（1 atm）下易于执行，包括使用大量丁二烯和/或异戊二烯原料。

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来源
《Journal of the American Chemical Society》 |2018年第6期|2050-2053|共4页
作者
Andreu Tortajada; Ryo Ninokata; Ruben Martin;
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作者单位

Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology, Av. Països Catalans 16, 43007 Tarragona, Spain;

Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology, Av. Països Catalans 16, 43007 Tarragona, Spain;

Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology, Av. Països Catalans 16, 43007 Tarragona, Spain,ICREA, Passeig Lluïs Companys, 23, 08010 Barcelona, Spain;

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入库时间 2022-08-18 03:07:19

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2. Stereoselective synthesis of pentasubstituted 1,3-dienes via Ni-catalyzed reductive coupling of unsymmetrical internal alkynes [J] . Zhijun Zhou, Jiachang Chen, Herong Chen, Chemical science . 2020,第37期

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3. Photoredox Ni-Catalyzed Branch-Selective Reductive Coupling of Aldehydes with 1,3-Dienes [J] . Li Yan-Lin, Li Wen-Duo, Gu Zheng-Yang, ACS catalysis . 2020,第2期

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7. Ni-Catalyzed Site-Selective Dicarboxylation of 1,3-Dienes with CO2 [O] . -1

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Ni-Catalyzed Site-Selective Dicarboxylation of 1,3-Dienes with CO_2

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