A Kinetic Study of Selective Hydrogenation of Carbon Monoxide to C_2 Oxygenates on Rh-Mn-Li-Fe/SiO_2 Catalyst

Hongmei Yin; Yunjie Ding; Hongyuan Luo; Daiping He; Weimiao Chen; Zhiyong Ao; Liwu Lin

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A Kinetic Study of Selective Hydrogenation of Carbon Monoxide to C_2 Oxygenates on Rh-Mn-Li-Fe/SiO_2 Catalyst

机译：Rh-Mn-Li-Fe / SiO_2催化剂上一氧化碳选择性加氢生成C_2氧化物的动力学研究

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摘要

The kinetics of CO hydrogenation for the synthesis of C_2 oxygenates over Rh-Mn-Li-Fe/SiO_2 was investigated. Kinetic parameters for the formation of ethanol, acetaldehyde, C'2 oxygenates, methanol and methane were obtained. The activation energy. H_2 and CO dependence orders for ethanol and acetaldehyde formation differed greatly, the large difference seemed to imply that they were formed through different intermediates.

机译：研究了在Rh-Mn-Li-Fe / SiO_2上CO加氢合成C_2含氧化合物的动力学。获得了形成乙醇，乙醛，C'2氧化物，甲醇和甲烷的动力学参数。活化能。 H_2和CO对乙醇和乙醛形成的依赖顺序差异很大，差异很大似乎暗示它们是通过不同的中间体形成的。

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来源
《Journal of Natural Gas Chemistry》 |2003年第4期|p.233-236|共4页
作者
Hongmei Yin; Yunjie Ding; Hongyuan Luo; Daiping He; Weimiao Chen; Zhiyong Ao; Liwu Lin;
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作者单位

Natural Gas Utilization and Applied Catalysis Laboratory, Dalian Institute of Chemical Physics, The Chinese Academy of Sciences, Dalian 116023, China;

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收录信息美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
原文格式 PDF
正文语种 eng
中图分类化学;
关键词
carbon monoxide; hydrogenation; Rh-Mn-Li-Fe/SiO_2 catalyst; C_2 oxygenates; kinetic;

机译：一氧化碳加氢Rh-Mn-Li-Fe / SiO_2催化剂C_2含氧化合物动力学;

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专利

1. A Kinetic Study of Selective Hydrogenation of Carbon Monoxide to C2 Oxygenates on Rh-Mn-Li-Fe/SiO2 Catalyst [J] . Hongmei Yin, Yunjie Ding, Hongyuan Luo, 天然气化学（英文版） . 2003,第004期

机译：Rh-Mn-Li-Fe / SiO2催化剂上一氧化碳选择性加氢生成C2氧化物的动力学研究
2. The Performance of C_2 Oxygenates Synthesis from Syngas over Rh-Mn-Li-Fe/SiO_2 Catalysts with Various Rh Loadings [J] . Hongmei Yin, Yunjie Ding, Hongyuan Luo, Energy & fuels . 2003,第6期

机译：Rh-Mn-Li-Fe / SiO_2催化剂在不同Rh负载下合成气合成C_2含氧化合物的性能
3. STUDIES OF HIGH SURFACE AREA PT/MOO3 AND PT/WO3 CATALYSTS FOR SELECTIVE HYDROGENATION REACTIONS .1. PREPARATION AND CHARACTERIZATION OF CATALYSTS BY X-RAY DIFFRACTION, TRANSMISSION ELECTRON MICROSCOPY, HYDROGEN CONSUMPTION AND CARBON MONOXIDE CHEMISO [J] . Hoangvan C., Zegaoui O. Applied Catalysis, A. General: An International Journal Devoted to Catalytic Science and Its Applications . 1995,第1期

机译：用于选择性加氢反应的高表面积PT / MOO3和PT / WO3催化剂的研究.1。 X射线衍射，透射电子显微镜，耗氢量和一氧化碳化学性质的催化剂的制备与表征
4. CuO/CeO2 Catalysts for Selective Oxidation of Carbon Monoxide in Excess Hydrogen [C] . International Conference on Rare Earth Research and Application; 2004; . 2004

机译：过量氢气中一氧化碳选择性氧化的CuO / CeO2催化剂
5. Oxygenate synthesis during carbon monoxide hydrogenation on cobalt copper Zinc oxzde-based catalysts [D] . Tsai, Yu-Tung 2011

机译：钴铜锌氧化锌基催化剂上一氧化碳加氢过程中的氧化物合成
6. Rate and selectivity hysteresis during the carbon monoxide hydrogenation over promoted Co/MnOx catalysts [O] . Yizhi Xiang, Libor Kovarik, Norbert Kruse -1

机译：促进型Co / MnOx催化剂在一氧化碳加氢过程中的速率和选择性滞后
7. A kinetic study on the adsorption and reaction of hydrogen over silica-supported ruthenium and silver-ruthenium catalysts during the hydrogenation of carbon monoxide [O] . VanderWiel, David Paul 1998

机译：一氧化碳加氢过程中氢在二氧化硅负载的钌和银-钌催化剂上吸附和反应的动力学研究
8. Kinetic study on the adsorption and reaction of hydrogen over silica-supported ruthenium and silver-ruthenium catalysts during the hydrogenation of carbon monoxide [R] . VanderWiel, D. P. 1999

机译：二氧化碳加氢过程中二氧化硅负载钌和银 - 钌催化剂上氢的吸附和反应动力学研究

A Kinetic Study of Selective Hydrogenation of Carbon Monoxide to C_2 Oxygenates on Rh-Mn-Li-Fe/SiO_2 Catalyst

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