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Spatially and temporally resolved spectral emission of laser-induced plasmas confined by cylindrical cavities

机译:圆柱腔限制的激光诱导等离子体的时空分辨光谱发射

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摘要

Laser-induced plasmas generated on pure copper samples in air with and without the presence of cylindrical cavities were investigated using spatially and temporally resolved spectroscopic measurements. The cylindrical cavities with variable diameters (3, 4 and 5 mm) and variable heights (1, 2, and 3 mm) were fabricated in quartz glass and placed on the sample surface and around the focused laser beam. Compared with plasmas generated without the cavity, the spectral emission intensities of plasmas generated with cylindrical cavities were enhanced after several microseconds, and the enhanced emission regions moved to higher locations above the sample with time. Plasma spatial and temporal emission was influenced by cavity diameter. As the diameter increased from 3 to 5 mm, the spectral emission was enhanced later in time and the enhancement became weaker. Plasma spatial and temporal emission was not significantly influenced by cavity height if the cavity was higher than the vapor plume. Shock wave theory was utilized to explain the observed phenomena.
机译:使用空间和时间分辨光谱测量方法研究了在有和没有圆柱孔的情况下在空气中的纯铜样品上产生的激光诱导等离子体。直径可变(3、4和5毫米)和高度可变(1、2和3毫米)的圆柱形空腔是用石英玻璃制成的,并放置在样品表面和聚焦的激光束周围。与没有空腔的等离子体相比,圆柱形空腔产生的等离子体的光谱发射强度在几微秒后有所增强,并且增强的发射区域会随时间移动到样品上方的较高位置。等离子体的时空发射受腔直径的影响。随着直径从3毫米增加到5毫米,光谱发射会在稍后时间增强,增强作用变弱。如果空腔比蒸气羽流高,则等离子体的空间和时间发射不受空腔高度的显着影响。冲击波理论被用来解释观察到的现象。

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  • 来源
    《Journal of Analytical Atomic Spectrometry》 |2014年第11期|2127-2135|共9页
  • 作者单位

    State Key Lab of Power Systems, Department of Thermal Engineering, Tsinghua-BP Clean Energy Center, Tsinghua University, Beijing, 100084, China;

    State Key Lab of Power Systems, Department of Thermal Engineering, Tsinghua-BP Clean Energy Center, Tsinghua University, Beijing, 100084, China;

    Lawrence Berkeley National Laboratory, University of California, Berkeley, California,94720, USA;

    Lawrence Berkeley National Laboratory, University of California, Berkeley, California,94720, USA;

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