Development of North American Emission Inventories for Air Quality Modeling under Climate Change

摘要

An assessment of how future climate change will impact regional air quality requires projecting emissions many decades into the future in a consistent manner. An approach that integrates the impact of both the current regulations and the longer-term national and global trends is developed to construct an emissions inventory (EI) for North America for the mid-century in support of a regional modeling study of ozone and particulate matter (PM) less than or equal to 2.5 μm (PM_(2.5)). Because the time horizon of such a distant projection is beyond that of EIs used in typical modeling studies, it is necessary to identify a practical approach that allows the emission projections to account for emission controls and climatic and energy-use changes. However, a technical challenge arises because this requires integration of various different types of information with which emissions from human activities are associated. Often, emission information in global models has less detail and uses coarser spatiotem-poral resolution. The method developed here is based on data availability, spatiotemporal coverage and resolution,rnand future-scenario consistency (i.e., Intergovernmental Panel on Climate Change Special Report on Emissions Scenarios [IPCC SRES] A1B), and consists of two major steps: (1) near-future EI projection (to the year 2020), and (2) longer-term EI projection (to mid-century). The first step is based closely on the U.S. Environmental Protection Agency Clean Air Interstate Rule EI, the Environment Canada EI, as well estimates of Mexico's EI; whereas the second step follows approaches proposed by the El from the Integrated Model to Assess the Global Environment (IMAGE), developed by Netherlands's National Institute for Public Health and the Environment (RIVM). For the United States, the year-2050 emissions for nitrogen oxides (NO_X), sulfur dioxide (SO_2), PM_(2.5), anthropogenic volatile organic compounds (VOCs), and ammonia are projected to change by -55, -55, -30, -40, and + 20%, respectively, compared with 2001. NO_X and SO_2 emission changes are very similar in total amount but different in sectoral contribution. The projected emission trends for Canada and Mexico differ considerably. After taking into account the modeled climate changes, biogenic VOC emission increases from three countries overwhelm the decreases in anthropogenic VOC emissions, leading to a net small increase (～2%) in overall VOC emissions.