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Optical Manipulation of Nano Materials under Quantum Mechanical Resonance Conditions

机译:量子机械共振条件下纳米材料的光学操纵

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We make a theoretical study about the laser-induced radiation force exerted on nano materials under a quantum mechanical resonance condition of electronic systems confined in them. In our recent study [ 1 ], we have clarified that the remarkable effects of the electronic resonance appear in the radiation force on the small object whose size is much smaller than the light wavelength; (A) the acceleration on the object gets larger as the size decreases, (B) the peaks with less heat appear in the force spectra even under the resonance condition, (C) the peak position sensitively varies with the nanoscale-size changes. These are useful for the optical manipulation to precisely control the mechanical motions of nano materials. In this paper, toward the experiment to verify the above results, we discuss the dependence of the mechanical motion of nano objects on the width of the incident laser light, and on the diffusion and friction effects assuming that they are floating in the superfiuid helium-4 with the cryogenic condition where the electronic resonance effects become conspicuous. The results of calculations show that the particular nano objects, whose resonance energy corresponds to the center frequency of incident laser, can move away from others over macroscopic distance beyond diffusion length. This means that we can observe the distribution of sizes and qualities of nano objects as a macroscopic spatial distribution of them if we prepare appropriate conditions of incident light. We call this new technique 'Nano Optical Chro-matography (NOC).'
机译:我们对限制在其中的电子系统在量子力学共振条件下施加在纳米材料上的激光诱导的辐射力进行了理论研究。在我们最近的研究中[1],我们已经弄清了电子共振的显着影响出现在对尺寸远小于光波长的小物体的辐射力上。 (A)随着尺寸减小,物体上的加速度变大;(B)即使在共振条件下,力谱中也会出现热量较少的峰;(C)峰位置随纳米级尺寸的变化而敏感地变化。这些对于光学操作以精确控制纳米材料的机械运动很有用。在本文中,为了验证上述结果,我们讨论了纳米物体的机械运动对入射激光宽度的依赖性,以及假设它们漂浮在超流体氦中的扩散和摩擦效应,图4是在低温条件下电子共振效应显着的情况。计算结果表明,特定的纳米物体的共振能量对应于入射激光的中心频率,可以在超过扩散长度的宏观距离上远离其他物体。这意味着,如果准备适当的入射光条件,我们可以观察到纳米物体的大小和质量分布,作为它们的宏观空间分布。我们称这种新技术为“纳米光学色谱法(NOC)”。

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