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Airborne Quantification of Methane Emissions over the Four Corners Region

机译:四个角落区域的甲烷排放的航空量化

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摘要

Methane (CH_4) is a potent greenhouse gas and the primary component of natural gas. The San Juan Basin (SJB) is one of the largest coal-bed methane producing regions in North America and, including gas production from conventional and shale sources, contributed 〜2% of U.S. natural gas production in 2015. In this work, we quantify the CH_4 flux from the SJB using continuous atmospheric sampling from aircraft collected during the TOP-DOWN2015 field campaign in April 2015. Using five independent days of measurements and the aircraft-based mass balance method, we calculate an average CH_4 flux of 0.54 ± 0.20 Tg yr~(-1) (lσ), in close agreement with the previous space-based estimate made for 2003-2009. These results agree within error with the U.S. EPA gridded inventory for 2012. These flights combined with the previous satellite study suggest CH_4 emissions have not changed. While there have been significant declines in natural gas production between measurements, recent increases in oil production in the SJB may explain why emission of CH_4 has not declined. Airborne quantification of outcrops where seepage occurs are consistent with ground-based studies that indicate these geological sources are a small fraction of the basin total (0.02-0.12 Tg yr~(-1)) and cannot explain basinwide consistent emissions from 2003 to 2015.
机译:甲烷(CH_4)是强温室气体,是天然气的主要成分。圣胡安盆地(SJB)是北美最大的煤层气生产区之一,其中包括常规气和页岩气的天然气产量,占2015年美国天然气产量的2%。在这项工作中,我们进行了量化使用在2015年4月TOP-DOWN2015野战期间收集的飞机的连续大气采样,从SJB获得CH_4通量。使用五天的独立测量时间和基于飞机的质量平衡方法,我们计算出平均CH_4通量为0.54±0.20 Tg yr〜(-1)(lσ),与先前对2003-2009年进行的天基估计非常吻合。这些结果与美国EPA 2012年的网格化清单存在误差。这些飞行与先前的卫星研究相结合,表明CH_4的排放没有改变。尽管两次测量之间的天然气产量已显着下降,但SJB中石油产量的近期增长可能可以解释为什么CH_4的排放没有下降。露头发生渗漏的空中量化与地面研究一致,这些研究表明这些地质源仅占盆地总数的一小部分(0.02-0.12 Tg yr〜(-1)),无法解释2003年至2015年整个盆地的一致排放量。

著录项

  • 来源
    《Environmental Science & Technology》 |2017年第10期|5832-5837|共6页
  • 作者单位

    Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, Michigan 48109, United States;

    Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, Michigan 48109, United States;

    Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, Michigan 48109, United States;

    Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder, Colorado 80305, United States;

    Scientific Aviation, Boulder, Colorado 80301;

    United States,Department of Land, Air, & Water Resources, University of California Davis, Davis, California 95616, United States;

    Department of Land, Air, & Water Resources, University of California Davis, Davis, California 95616, United States;

    Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder, Colorado 80305, United States;

    NOAA Earth System Research Laboratory, Boulder, Colorado 80305, United States;

    Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder, Colorado 80305, United States;

    Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder, Colorado 80305, United States;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
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  • 入库时间 2022-08-17 13:57:36

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