Potential for developing independent daytime/nighttime LUR models based on short-term mobile monitoring to improve model performance

摘要

Land use regression model (LUR) is a widespread method for predicting air pollution exposure. Few studies have explored the performance of independently developed daytime/nighttime LUR models. In this study, fine particulate matter (PM2.5), inhalable particulate matter (PM10), and nitrogen dioxide (NO2) concentrations were measured by mobile monitoring during non-heating and heating seasons in Taiyuan. Pollutant concentrations were higher in the nighttime than the daytime, and higher in the heating season than the non-heating season. Daytime/nighttime and full-day LUR models were developed and validated for each pollutant to examine variations in model performance. Adjusted coefficients of determination (adjusted R-2) for the LUR models ranged from 0.53-0.87 (PM2.5), 0.53-0.85 (PM10), and 0.33-0.67 (NO2). The performance of the daytime/nighttime LUR models for PM2.5 and PM10 was better than that of the full-day models according to the results of model adjusted R-2 and validation R-2. Consistent results were confirmed in the non-heating and heating seasons. Effectiveness of developing independent daytime/nighttime models for NO2 to improve performance was limited. Surfaces based on the daytime/nighttime models revealed variations in concentrations and spatial distribution. In conclusion, the independent development of daytime/nighttime LUR models for PM2.5/PM10 has the potential to replace full-day models for better model performance. The modeling strategy is consistent with the residential activity patterns and contributes to achieving reliable exposure predictions for PM2.5 and PM10. Nighttime could be a critical exposure period, due to high pollutant concentrations. (C) 2020 Elsevier Ltd. All rights reserved.