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首页> 外文期刊>Atmospheric Chemistry and Physics Discussions >Spectral optical properties of long-range transport Asian dust and pollution aerosols over Northeast Asia in 2007 and 2008
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Spectral optical properties of long-range transport Asian dust and pollution aerosols over Northeast Asia in 2007 and 2008

机译:2007年和2008年东北亚远程运输亚洲粉尘和污染气溶胶的光谱光学特性

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As a part of the IGAC (International Global Atmospheric Chemistry) Mega-cities program, aerosol physical and optical properties were continuously measured from March 2007 to March 2008 at an urban site (37.57° N, 126.94° E) in Seoul, Korea. Spectral optical properties of long-range transported Asian dust and pollution aerosols have been investigated based on the year long measurement data. Optically measured black carbon/thermally measured elemental carbon (BC/EC) ratio showed clear monthly variation with high values in summer and low values in winter mainly due to the enhancement of light attenuation by the internal mixing of EC. Novel approach has been suggested to retrieve the spectral light absorption coefficient (babs) from Aethalometer raw data by using BC/EC ratio. Mass absorption efficiency, abs (=babs/EC) at 550 nm was determined to be 9.01.3, 8.91.5, 9.52.0, and 10.31.7 m2 g?1 in spring, summer, fall, and winter, respectively with an annual mean of 9.41.8 m2 g?1. Threshold values to classify severe haze events were suggested in this study. Increasing trend of aerosol single scattering albedo (SSA) with wavelength was observed during Asian dust events while little spectral dependence of SSA was observed during long-range transport pollution (LTP) events. Satellite aerosol optical thickness (AOT) and Hysplit air mass backward trajectory analyses as well as chemical analysis were performed to characterize the dependence of spectral optical properties on aerosol type. Results from this study can provide useful information for studies on regional air quality and aerosol's effects on climate change.
机译:作为IGAC(国际全球大气化学)的一部分Mega-Cities计划,从2007年3月到2008年3月在韩国首尔的城市网站(37.57°N,126.94°E)中持续测量气溶胶物理和光学性质。基于年度的测量数据研究了远程运输的亚洲灰尘和污染气溶胶的光谱光学性能。光学测量的黑碳/热测量的元素碳(BC / EC)比率在夏季夏季和低值中显示出明显的月度变化,主要是由于EC的内部混合增强了光衰减。已经建议通过使用BC / EC比来检索来自聚体仪原始数据的光谱光吸收系数(Babs)。在550nm处的质量吸收效率,Abs(= Babs / EC)分别测定为9.01.3,8.91.5,9.52.0和10.31.7m2 g?1分别在春季,夏季,秋季和冬季年平均值为9.41.8 m2 g?1。在本研究中提出了分类严重阴霾事件的阈值。在亚洲粉尘事件期间观察到具有波长的气溶胶单散射玻璃玻璃(SSA)的趋势,而在远程运输污染(LTP)事件期间观察到SSA的小光谱依赖性。进行卫星气溶胶光学厚度(AOT)和Hysplit空气质量向后轨迹分析以及化学分析,以表征光谱光学性质对气溶胶型的依赖性。本研究的结果可以提供有关区域空气质量和气溶胶对气候变化影响的有用信息。

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