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Impacts of future climate change and effects of biogenic emissions on surface ozone and particulate matter concentrations in the United States

机译:未来气候变化对未来气候变化的影响和生物发射对地表臭氧和颗粒物质浓度的影响

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Simulations of present and future average regional ozone and PM2.5 concentrations over the United States were performed to investigate the potential impacts of global climate change and emissions on regional air quality using CMAQ. Various emissions and climate conditions with different biogenic emissions and domain resolutions were implemented to study the sensitivity of future air quality trends from the impacts of changing biogenic emissions. A comparison of GEOS-Chem and CMAQ was performed to investigate the effect of downscaling on the prediction of future air quality trends. For ozone, the impacts of global climate change are relatively smaller when compared to the impacts of anticipated future emissions reduction, except for the Northeast area, where increasing biogenic emissions due to climate change have stronger positive effects (increases) to the regional ozone air quality. The combination effect from both climate change and emission reductions leads to approximately a 10 % or 5 ppbv decrease of the maximum daily average eight-hour ozone (MDA8) over the Eastern United States. For PM2.5, the impacts of global climate change have shown insignificant effect, where as the impacts of anticipated future emissions reduction account for the majority of overall PM2.5 reductions. The annual average 24-h PM2.5 of the future-year condition was found to be about 40 % lower than the one from the present-year condition, of which 60 % of its overall reductions are contributed to by the decrease of SO4 and NO3 particulate matters. Changing the biogenic emissions model increases the MDA8 ozone by about 5–10 % or 3–5 ppbv in the Northeast area. Conversely, it reduces the annual average PM2.5 by 5 % or 1.0 μg m3 in the Southeast region.
机译:在美国的目前和未来普通区域臭氧和PM2.5浓度的模拟,探讨了使用CMAQ的全球气候变化和排放对区域空气质量的潜在影响。实施了不同生物排放和域决议的各种排放和气候条件,以研究从改变生物排放的影响的未来空气质量趋势的敏感性。进行了Geos-Chem和CMAQ的比较,以研究令人抵制对未来空气质量趋势预测的影响。对于臭氧,与预期未来排放减少的影响相比,全球气候变化的影响相对较小,除了东北地区外,除了气候变化导致的生物发射增加,对区域臭氧空气质量的较强的积极影响(增加) 。气候变化和排放减少的组合效应导致美国东部地区最高八小时臭氧(MDA8)的最大每日八小时臭氧减少约10%或5 PPBV。对于PM2.5来说,全球气候变化的影响表现出微不足道的效果,因为预期未来排放减少的影响占总PM2.5减少的减少。未来年度条件的年平均24小时PM2.5比目前一年条件低约40%,其中60%的整体减少是由SO4的减少贡献no3微粒问题。改变生物发射模型将MDA8臭氧增加约5-10%或3-5个PPBV在东北地区。相反,它将年平均PM2.5减少到东南部地区5%或1.0微克M3。

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