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Inverse modelling of CH4 emissions for 2010–2011 using different satellite retrieval products from GOSAT and SCIAMACHY

机译:2010 - 2011年CH4排放的逆建模使用Gosat和Sciamachy的不同卫星检索产品

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At the beginning of 2009 new space-borne observations of dry-air column-averaged mole fractions of atmospheric methane (XCH4) became available from the Thermal And Near infrared Sensor for carbon Observations–Fourier Transform Spectrometer (TANSO-FTS) instrument on board the Greenhouse Gases Observing SATellite (GOSAT). Until April 2012 concurrent {methane (CH4) retrievals} were provided by the SCanning Imaging Absorption spectroMeter for Atmospheric CartograpHY (SCIAMACHY) instrument on board the ENVironmental SATellite (ENVISAT). The GOSAT and SCIAMACHY XCH4 retrievals can be compared during the period of overlap. We estimate monthly average CH4 emissions between January 2010 and December 2011, using the TM5-4DVAR inverse modelling system. In addition to satellite data, high-accuracy measurements from the Cooperative Air Sampling Network of the National Oceanic and Atmospheric Administration Earth System Research Laboratory (NOAA ESRL) are used, providing strong constraints on the remote surface atmosphere. We discuss five inversion scenarios that make use of different GOSAT and SCIAMACHY XCH4 retrieval products, including two sets of GOSAT proxy retrievals processed independently by the Netherlands Institute for Space Research (SRON)/Karlsruhe Institute of Technology (KIT), and the University of Leicester (UL), and the RemoTeC "Full-Physics" (FP) XCH4 retrievals available from SRON/KIT. The GOSAT-based inversions show significant reductions in the root mean square (rms) difference between retrieved and modelled XCH4, and require much smaller bias corrections compared to the inversion using SCIAMACHY retrievals, reflecting the higher precision and relative accuracy of the GOSAT XCH4. Despite the large differences between the GOSAT and SCIAMACHY retrievals, 2-year average emission maps show overall good agreement among all satellite-based inversions, with consistent flux adjustment patterns, particularly across equatorial Africa and North America. Over North America, the satellite inversions result in a significant redistribution of CH4 emissions from North-East to South-Central United States. This result is consistent with recent independent studies suggesting a systematic underestimation of CH4 emissions from North American fossil fuel sources in bottom-up inventories, likely related to natural gas production facilities. Furthermore, all four satellite inversions yield lower CH4 fluxes across the Congo basin compared to the NOAA-only scenario, but higher emissions across tropical East Africa. The GOSAT and SCIAMACHY inversions show similar performance when validated against independent shipboard and aircraft observations, and XCH4 retrievals available from the Total Carbon Column Observing Network (TCCON).
机译:在2009年初开始,在碳观察 - 傅立叶变换光谱仪(TANSO-FTS)仪器上的热和近红外传感器中,可以获得大气甲烷(XCH4)的干燥空气柱平均摩尔分数的新空间甲烷(XCH4)的观察温室气体观察卫星(Gosat)。直到2012年4月,并发{甲烷(CH4)检索}由扫描成像吸收光谱仪提供环境卫星(Envisat)的大气制图(Sciamachy)仪器。可以在重叠期间比较Gosat和Sciamachy Xch4检索。我们使用TM5-4DVAR反转建模系统估计2010年1月至2011年12月之间的月平均CH4排放量。除了卫星数据外,还使用来自国家海洋和大气管理地球系统研究实验室(NOAA ESRL)的合作空气采样网络的高精度测量,为遥控表面大气提供强大的限制。我们讨论了五种反转情景,利用不同的Gosat和Sciamachy Xch4检索产品,包括由荷兰空间研究所(Sron)/ Karlsruhe技术研究所(Kit)和莱斯特大学独立处理的两套Gosat Proxy检索。 (UL)和Remotec“全物理”(FP)Xch4从Sron / Kit获得的检索。基于GOSAT的逆转显示出检索和建模的XCH4之间的根均线(RMS)差异的显着减少,并且与使用SCIMACHY检索的反演相比,需要更小的偏差校正,反映了GOSAT XCH4的更高精度和相对精度。尽管Gosat和Sciamachy检索之间存在巨大差异,但2年的平均排放图在所有卫星的反转中表现出整体良好的一致性,其中助焊剂调整模式一致,特别是赤道非洲和北美。在北美,卫星反转导致从美国东南到美国东北部的CH4排放量重新分配。该结果与最近的独立研究一致,表明系统地低估了从自然气体生产设施的自下而上库存中北美化石燃料源的CH4排放。此外,与NOAA的场景相比,所有四种卫星反转产生刚果盆地的较低的CH4势次,而是热带东非的较高排放。当验证独立的船上和飞机观察时,Gosat和Sciamachy逆势显示出类似的性能,以及可从总碳柱观察网络(TCCON)的XCH4检索。
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