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A high-resolution emission inventory of primary pollutants for the Huabei region, China

机译:中国淮北地区初级污染物的高分辨率排放清单

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Huabei, located between 32° N and 42° N, is part of eastern China and includes administratively the Beijing and Tianjin Municipalities, Hebei and Shanxi Provinces, and Inner-Mongolia Autonomous Region. Over the past decades, the region has experienced dramatic changes in air quality and climate, and has become a major focus of environmental research in China. Here we present a new inventory of air pollutant emissions in Huabei for the year 2003 developed as part of the project Influence of Pollution on Aerosols and Cloud Microphysics in North China (IPAC-NC). Our estimates are based on data from the statistical yearbooks of the state, provinces and local districts, including major sectors and activities of power generation, industrial energy consumption, industrial processing, civil energy consumption, crop straw burning, oil and solvent evaporation, manure, and motor vehicles. The emission factors are selected from a variety of literature and those from local measurements in China are used whenever available. The estimated total emissions in the Huabei administrative region in 2003 are 4.73 Tg SO2, 2.72 Tg NOx (in equivalent NO2), 1.77 Tg VOC, 24.14 Tg CO, 2.03 Tg NH3, 4.57 Tg PM10, 2.42 Tg PM2.5, 0.21 Tg EC, and 0.46 Tg OC. For model convenience, we consider a larger Huabei region with Shandong, Henan and Liaoning Provinces included in our inventory. The estimated total emissions in the larger Huabei region in 2003 are: 9.55 Tg SO2, 5.27 Tg NOx (in equivalent NO2), 3.82 Tg VOC, 46.59 Tg CO, 5.36 Tg NH3, 10.74 Tg PM10, 5.62 Tg PM2.5, 0.41 Tg EC, and 0.99 Tg OC. The estimated emission rates are projected into grid cells at a horizontal resolution of 0.1° latitude by 0.1° longitude. Our gridded emission inventory consists of area sources, which are classified into industrial, civil, traffic, and straw burning sectors, and large industrial point sources, which include 345 sets of power plants, iron and steel plants, cement plants, and chemical plants. The estimated regional NO2 emissions are about 2–3% (administrative Huabei region) or 5% (larger Huabei region) of the global anthropogenic NO2 emissions. We compare our inventory (IPAC-NC) with the global emission inventory EDGAR-CIRCE and the Asian emission inventory INTEX-B. Except for a factor of 3 lower EC emission rate in comparison with INTEX-B, the biases of the total emissions of most primary air pollutants in Huabei estimated in our inventory, with respect to EDGAR-CIRCE and INTEX-B, generally range from ?30% to +40%. Large differences up to a factor of 2–3 for local emissions in some areas (e.g. Beijing and Tianjin) are found. It is recommended that the inventories based on the activity rates and emission factors for each specific year should be applied in future modeling work related to the changes in air quality and atmospheric chemistry over this region.
机译:淮北位于32°N和42°N之间,是中国东部的一部分,包括行政上的北京和天津市,河北和山西省,内部蒙古自治区。在过去几十年中,该地区经历了空气质量和气候的巨大变化,并已成为中国环境研究的重点。在这里,我们为2003年开发的2003年乌贝的空气污染物排放量新库存是污染对华北地区气溶胶和云微生物的影响的一部分。我们的估计是基于国家,省和地方地区统计年鉴的数据,包括发电,工业能源消费,工业加工,民能量消耗,作物秸秆燃烧,油和溶剂蒸发,粪肥,粪肥,粪便,和机动车辆。排放因子选自各种文献,每当可用时,使用来自中国的局部测量的因素。估计2003年华湾行政区域的总排放量为4.73 TG SO2,2.72 TG NOx(相当于NO2),1.77 TG VOC,24.14 TG CO,2.03 TG NH3,4.57 TG PM10,2.42 TG PM2.5,0.21 TG PM2.5,0.21 TG EC和0.46 tg oc。对于型号便利,我们考虑了与山东,河南和辽宁省内的较大的华北地区。 2003年较大的华北地区估计的总排放是:9.55 TG SO2,5.27 TG NOx(相当于NO2),3.82 TG VOC,46.59 TG CO,5.36 TG NH3,10.74 TG PM10,5.62 TG PM2.5,0.41 TG EC,0.99 TG OC。估计的排放率以0.1°纬度的水平分辨率投射到网格细胞中,经度0.1°。我们的网格排放库存包括区域来源,分为工业,公民,交通和稻草燃烧部门以及大型工业点来源,包括345套发电厂,钢铁厂,水泥厂和化工厂。所估计的区域NO2排放是对全球人为NO2排放的2-3%(行政华北区域)或5%(较大华北区域)。我们将库存(IPAC-NC)与全球排放库存Edgar-Circe和亚洲排放库存Intex-B进行比较。除Intex-B相比,除了INTEX-B相比,除了3较低的EC排放率较小,在我们的库存中估计,在我们的库存中估计,关于Edgar-Circe和Intex-B,估计的大多数原发性空气污染物的总排放的偏差通常是速度的? 30%至+ 40%。在发现某些地区(例如北京和天津)的当地排放量大于2-3倍。建议根据该地区的空气质量和大气化学变化的未来建模工作中应用基于每个特定年度的活动率和排放因子的库存。

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