首页> 外文期刊>Atmospheric Chemistry and Physics Discussions >Microphysical characterization of long-range transported biomass burning particles from North America at three EARLINET stations
【24h】

Microphysical characterization of long-range transported biomass burning particles from North America at three EARLINET stations

机译:三个耳线站北美远程运输生物质燃烧颗粒的微神科表征

获取原文
           

摘要

Strong events of long-range transported biomass burning aerosol were detected during July?2013 at three EARLINET (European Aerosol Research Lidar Network) stations, namely Granada (Spain), Leipzig (Germany) and Warsaw (Poland). Satellite observations from MODIS (Moderate Resolution Imaging Spectroradiometer) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) instruments, as well as modeling tools such as HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) and NAAPS (Navy Aerosol Analysis and Prediction System), have been used to estimate the sources and transport paths of those North American forest fire smoke particles. A multiwavelength Raman lidar technique was applied to obtain vertically resolved particle optical properties, and further inversion of those properties with a regularization algorithm allowed for retrieving microphysical information on the studied particles. The results highlight the presence of smoke layers of 1–2?km thickness, located at about 5?km?a.s.l. altitude over Granada and Leipzig and around 2.5?km?a.s.l. at Warsaw. These layers were intense, as they accounted for more than 30?% of the total AOD (aerosol optical depth) in all cases, and presented optical and microphysical features typical for different aging degrees: color ratio of lidar ratios (LR532?∕?LR355) around 2, α-related ?ngstr?m exponents of less than 1, effective radii of 0.3?μm and large values of single scattering albedos (SSA), nearly spectrally independent. The intensive microphysical properties were compared with columnar retrievals form co-located AERONET (Aerosol Robotic Network) stations. The intensity of the layers was also characterized in terms of particle volume concentration, and then an experimental relationship between this magnitude and the particle extinction coefficient was established.
机译:7月份在七月举行的长期运输生物量燃烧气溶胶的强烈事件2013年在三个耳坠(欧洲气溶胶研究激光雷达网络)站,即格拉纳达(西班牙),莱比锡(德国)和华沙(波兰)。来自MODIS(中等分辨率成像分光镜)和卡利波(具有正交偏振的云气旋LIDAR)的卫星观察,以及诸如HYSPLIT(混合单粒子Lagrangian集成轨迹)和赤行的建模工具(海军气溶胶分析和预测系统) ,已被用来估计这些北美森林火灾烟雾颗粒的来源和运输路径。施加多波长拉曼利达技术以获得垂直分辨的粒子光学性质,并进一步反演这些性质,其允许检索研究颗粒上的微神科信息的正则化算法。结果突出了1-2 km厚度的烟层的存在,位于约5Ωkm?a .l。高度超过格拉纳达和莱比锡和大约2.5英里?A.S.L。在华沙。这些层是激烈的,因为它们在所有情况下占总AOD(气溶胶光学深度)的30多个超过30?%,并且呈现出不同老化程度的光学和微手术特征:LIDAR比的颜色比(LR532?/?LR355 )大约2,α相关的?NGSTRαM指数小于1,有效的半径为0.3ΩΩΩmm,单次散射玻璃玻璃(SSA)的大值,几乎是光谱无关的。将密集的微神科性质与共同定位的AeroNet(气溶胶机器人网络)站进行比较。层的强度还表征在颗粒体积浓度方面,然后建立了该幅度与颗粒消光系数之间的实验关系。
获取原文

客服邮箱:kefu@zhangqiaokeyan.com

京公网安备:11010802029741号 ICP备案号:京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有
  • 客服微信

  • 服务号