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Apparent dust size discrepancy in aerosol reanalysis in north African dust after long-range transport

机译:在远程运输后北非尘埃在气溶胶再分析的明显灰尘差异

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North African dust reaches the southeastern United States every summer. Size-resolved dust mass measurements taken in Miami, Florida, indicate that more than one-half of the surface dust mass concentrations reside in particles with geometric diameters less than 2.1μm, while vertical profiles of micropulse lidar depolarization ratios show dust reaching above 4km during pronounced events. These observations are compared to the representation of dust in the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) aerosol reanalysis and closely related Goddard Earth Observing System model version?5 (GEOS-5) Forward Processing (FP) aerosol product, both of which assimilate satellite-derived aerosol optical depths using a similar protocol and inputs. These capture the day-to-day variability in aerosol optical depth well, in a comparison to an independent sun-photometer-derived aerosol optical depth dataset. Most of the modeled dust mass resides in diameters between 2 and 6μm, in contrast to the measurements. Model-specified mass extinction efficiencies equate light extinction with approximately 3?times as much aerosol mass, in this size range, compared to the measured dust sizes. GEOS-5 FP surface-layer sea salt mass concentrations greatly exceed observed values, despite realistic winds and relative humidities. In combination, these observations help explain why, despite realistic total aerosol optical depths, (1)?free-tropospheric model volume extinction coefficients are lower than those retrieved from the micro-pulse lidar, suggesting too-low model dust loadings in the free troposphere, and (2)?model dust mass concentrations near the surface can be higher than those measured. The modeled vertical distribution of dust, when captured, is reasonable. Large, aspherical particles exceeding the modeled dust sizes are also occasionally present, but dust particles with diameters exceeding 10μm contribute little to the measured total dust mass concentrations after such long-range transport. Remaining uncertainties warrant a further integrated assessment to confirm this study's interpretations.
机译:北非尘埃每年夏天到达美国东南部。在佛罗里达州迈阿密拍摄的尺寸分辨粉尘测量表明,表面粉尘质量浓度的大于一半以上的几何直径小于2.1μm的颗粒,而微孔激光雷达去极化比率的垂直轮廓显示出在4km以上的灰尘发音的事件。将这些观察结果与现代时代回顾性分析中的灰尘的代表进行了比较,版本2(Merra-2)气溶胶再分析和密切相关的戈达德地球观测系统模型版本?5(Geos-5)前进处理(FP )气溶胶产品,其中两者都使用类似的协议和输入来吸化卫星衍生的气溶胶光学深度。这些与独立的太阳光度计衍生的气溶胶光学深度数据集相比,这些捕获了气溶胶光学深度的日常变异性。与测量相比,大多数建模粉尘质量在2至6μm之间存在于2至6μm之间的直径。与测量的粉尘尺寸相比,模型特定质量消光效率在该尺寸范围内具有大约3倍的气溶胶质量的光消失。尽管现实的风和相对湿度,但Geos-5 FP表面层海盐质量浓度大大超过观察到的值。组合,这些观察结果有助于解释为什么,尽管现实的气溶胶光学深度,(1)?自由 - 对流层模型体积消光系数低于从微脉冲激光雷达检出的那些,表明自由对流层中的太低模型粉尘载荷(2)?表面附近的模型粉尘质量浓度可以高于测量的粉尘质量浓度。捕获时,灰尘的建模垂直分布是合理的。大型非球面颗粒超过建模粉尘尺寸也偶尔存在,但是直径超过10μm的粉尘颗粒对于这种远距离运输后测量的总粉尘质量浓度几乎没有贡献。剩余的不确定因素是进一步的综合评估,以确认这项研究的解释。

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