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A case study of aerosol scavenging in a biomass burning plume over eastern Canada during the 2011 BORTAS field experiment

机译:2011年Bortas Field实验期间加拿大东部燃烧羽流气溶胶清除案例

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We present measurements of a long-range smoke transport event recorded on 20–21 July 2011 over Halifax, Nova Scotia, Canada, during the Quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites (BORTAS-B) campaign. Ground-based Fourier transform spectrometers and photometers detected air masses associated with large wildland fires burning in eastern Manitoba and western Ontario. We investigate a plume with high trace gas amounts but low amounts of particles that preceded and overlapped at the Halifax site with a second plume with high trace gas loadings and significant amounts of particulate material. We show that the first plume experienced a meteorological scavenging event, but the second plume had not been similarly scavenged. This points to the necessity to account carefully for the plume history when considering long-range transport since simultaneous or near-simultaneous times of arrival are not necessarily indicative of either similar trajectories or meteorological history. We investigate the origin of the scavenged plume, and the possibility of an aerosol wet deposition event occurring in the plume ~ 24 h prior to the measurements over Halifax. The region of lofting and scavenging is only monitored on an intermittent basis by the present observing network, and thus we must consider many different pieces of evidence in an effort to understand the early dynamics of the plume. Through this discussion we also demonstrate the value of having many simultaneous remote-sensing measurements in order to understand the physical and chemical behaviour of biomass burning plumes.
机译:我们在2011年7月20日至21日举办的远程烟雾运输活动的测量在加拿大新斯科舍省的哈利法克斯(Nova Scotia),在使用飞机和卫星(Bortas-B)上量化北方森林火灾对地球氧化剂的影响活动。基于地面的傅里叶变换光谱仪和光度计检测到与曼尼托巴省东部和安大略省西部燃烧的大型野外火灾相关的空气肿块。我们研究了具有高痕量气体的羽流,但在哈利法克斯位点之前并重叠的颗粒具有较低的颗粒,其具有高痕量气体载体和大量的颗粒材料。我们表明,第一次羽流经历了气象清除事件,但第二羽羽流并未类似地清除。这指出了在考虑远程运输时仔细考虑羽流历史的必要性,因为同时或接近同时到达时不一定指示具有类似的轨迹或气象史。我们研究了清除羽流的起源,在哈利法克斯的测量之前,在羽毛〜24小时内发生气溶胶湿沉积事件的可能性。 Lofting和Pravenging的区域仅在目前的观察网络间歇性地监测,因此我们必须考虑许多不同的证据,以了解羽流的早期动态。通过该讨论,我们还展示了具有许多同步遥感测量的值,以便理解生物质燃烧羽毛的物理和化学行为。
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