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Using a combined power law and log-normal distribution model to simulate particle formation and growth in a mobile aerosol chamber

机译:使用组合的电力法和日志正态分布模型来模拟移动气溶胶室中的粒子形成和生长

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We present the combined power law and log-normal distribution (PL+LN) model, a computationally efficient model to be used in simulations where the particle size distribution cannot be accurately represented by log-normal distributions, such as in simulations involving the initial steps of aerosol formation, where new particle formation and growth occur simultaneously, or in the case of inverse modeling. The model was evaluated against highly accurate sectional models using input parameter values that reflect conditions typical to particle formation occurring in the atmosphere and in vehicle exhaust. The model was tested in the simulation of a particle formation event performed in a mobile aerosol chamber at M?kel?nkatu street canyon measurement site in Helsinki, Finland. The number, surface area, and mass concentrations in the chamber simulation were conserved with the relative errors lower than 2?% using the PL+LN model, whereas a moment-based log-normal model and sectional models with the same computing time as with the PL+LN model caused relative errors up to 17 and 79?%, respectively.
机译:我们介绍了组合的电力法和日志正态分布(PL + LN)模型,用于模拟的计算有效模型,其中粒度分布不能被记录正态分布准确表示,例如涉及初始步骤的模拟气溶胶形成,其中新的颗粒形成和生长同时发生,或在逆建模的情况下发生。使用反映在大气中发生的颗粒形成和车辆排气的颗粒形成的输入参数值来评估模型的高度精确的截面模型。该模型在M赫尔辛基,芬兰赫尔辛基的移动气溶胶室中进行的粒子形成事件的模拟进行了测试。腔室模拟中的数量,表面积和质量浓度随PL + LN模型的相对误差被保守,而使用PL + LN型号的相对误差,而基于矩的日志正常模型和具有相同计算时间的截面模型PL + LN模型分别导致相对误差高达17和79?%。

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