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Spatial distribution of aerosol microphysical and optical properties and direct radiative effect from the China Aerosol Remote Sensing Network

机译:气溶胶微物理和光学性质的空间分布,中国气溶胶遥感网络直接辐射效果

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Multi-year observations of aerosol microphysical and optical properties, obtained through ground-based remote sensing at 50 China Aerosol Remote Sensing Network (CARSNET) sites, were used to characterize the aerosol climatology for representative remote, rural, and urban areas over China to assess effects on climate. The annual mean effective radii for total particles (ReffT) decreased from north to south and from rural to urban sites, and high total particle volumes were found at the urban sites. The aerosol optical depth at 440nm (AOD440?nm) increased from remote and rural sites (0.12) to urban sites (0.79), and the extinction ?ngstr?m exponent (EAE440–870nm) increased from 0.71 at the arid and semi-arid sites to 1.15 at the urban sites, presumably due to anthropogenic emissions. Single-scattering albedo (SSA440?nm) ranged from 0.88 to 0.92, indicating slightly to strongly absorbing aerosols. Absorption AOD440?nm values were 0.01 at the remote sites versus 0.07 at the urban sites. The average direct aerosol radiative effect (DARE) at the bottom of atmosphere increased from the sites in the remote areas (?24.40Wm?2) to the urban areas (?103.28Wm?2), indicating increased cooling at the latter. The DARE for the top of the atmosphere increased from ?4.79Wm?2 at the remote sites to ?30.05Wm?2 at the urban sites, indicating overall cooling effects for the Earth–atmosphere system. A classification method based on SSA440?nm, fine-mode fraction (FMF), and EAE440–870?nm showed that coarse-mode particles (mainly dust) were dominant at the rural sites near the northwestern deserts, while light-absorbing, fine-mode particles were important at most urban sites. This study will be important for understanding aerosol climate effects and regional environmental pollution, and the results will provide useful information for satellite validation and the improvement of climate modelling.
机译:通过在50个中国气溶胶遥感网络(Carsnet)地点的地面遥感的气溶胶微物理和光学性质的多年观测用于表征中国代表遥远,农村和城市地区的气溶胶气候学评估对气候的影响。总颗粒(REFFT)的年平均效半径从北部到南部和从农村到城市网站减少,在城市网站发现了高的总粒子量。 440nm(AOD440?NM)的气溶胶光学深度从远程和农村地点(0.12)增加到城市网站(0.79),灭绝?NGSTR?M指数(EAE440-870NM)从干旱和半干旱的0.71增加城市遗址的网站至1.15,可能是由于人为排放。单散射反玻璃(SSA440?NM)的范围为0.88至0.92,表明略微吸收气溶胶。在城市地点,远程站点的吸收AOD440?NM值为0.01。大气底部的平均直接气溶胶辐射效果(敢于)从偏远地区(?24.40WM?2)到城市地区(?103.28WM?2)的地点增加,表明后者的冷却增加。大气层的敢于从偏远地点的4.79WM?2到4.79WM?2在城市网站上的30.05WM?2,表明地球大气系统的整体冷却效果。基于SSA440的分类方法,微量模式分数(FMF)和EAE440-870?NM表明,粗型颗粒(主要是灰尘)在西北沙漠附近的农村地点占主导地位,而光吸收,细腻 - Mode粒子在大多数城市网站都很重要。本研究对于了解气溶胶气候影响和区域环境污染至关重要,结果将为卫星验证和改善气候建模提供有用的信息。
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