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Aerosol optical properties in the North China Plain during HaChi campaign: an in-situ optical closure study

机译:Hachi Campaign期间华北平原气溶胶光学特性:原位光学闭合研究

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The largest uncertainty in the estimation of climate forcing stems from atmospheric aerosols. In early spring and summer of 2009, two periods of in-situ measurements on aerosol physical and chemical properties were conducted within the HaChi (Haze in China) project at Wuqing, a town between Beijing and Tianjin in the North China Plain (NCP). Aerosol optical properties, including the scattering coefficient (sp), the hemispheric back scattering coefficient (bsp), the absorption coefficient (ap), as well as the single scattering albedo (ω), are presented. The diurnal and seasonal variations are analyzed together with meteorology and satellite data. The mean values of sp, 550 nm of the dry aerosol in spring and summer are 280253 and 379251 Mm?1, respectively. The average ap for the two periods is respectively 4738 and 4327 Mm?1. The mean values of at the wavelength of 637 nm are 0.820.05 and 0.860.05 for spring and summer, respectively. The relative high levels of sp and bsp are representative of the regional aerosol pollution in the NCP. Pronounced diurnal cycle of $sp, ap and ω are found, mainly influenced by the evolution of boundary layer and the accumulation of local emissions during nighttime. The pollutants transported from the southwest of the NCP are more significant than that from the two megacities, Beijing and Tianjin, in both spring and summer. An optical closure experiment is conducted to better understand the uncertainties of the measurements. Good correlations (R0.98) are found between the values measured by the nephelometer and the values calculated with a modified Mie model. The Monte Carlo simulation shows an uncertainty of about 30 % for the calculations. Considering all possible uncertainties of measurements, calculated sp and bsp agree well with the measured values, indicating a stable performance of instruments and thus reliable aerosol optical data.
机译:估计气候迫使源于大气气溶胶的最大不确定性。在2009年初的春季和夏季,在武清的Hachi(中国阴霾中)在北京市平原(NCP)之间的一个城镇的Hachi(中国雾霾)项目中进行了两次原位测量。提出了气溶胶光学性质,包括散射系数(SP),半球背散射系数(BSP),吸收系数(AP)以及单散射玻璃玻璃(ω)。与气象和卫星数据一起分析昼夜和季节变化。 Sp的平均值,春季和夏季的干气溶胶550nm分别为280253和379251mm?1。两个时段的平均AP分别为4738和4327mm?1。春季和夏季分别为637nm波长637nm的平均值为0.820.05和0.860.05。 SP和BSP的相对高水平代表NCP中的区域气溶胶污染。发现的$ SP,AP和ω的明显昼夜周期,主要受边界层演变的影响和夜间局部排放的积累。从NCP西南部运输的污染物比春夏的两种兆瓦,北京和天津更重要。进行光学闭合实验以更好地了解测量的不确定性。在浊度计测量的值和用修改的MIE模型计算的值之间找到良好的相关性(R> 0.98)。蒙特卡罗模拟显示计算的不确定性约为30%。考虑到测量的所有可能的不确定性,计算的SP和BSP与测量值吻合良好,表明仪器的稳定性能,因此可靠的气溶胶光学数据。
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