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Simplifying the calculation of light scattering properties for black carbon fractal aggregates

机译:简化黑碳分形聚集体的光散射性能的计算

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Black carbon fractal aggregates have complicated shapes that make the calculation of their optical properties particularly computationally expensive. Here, a method is presented to estimate fractal aggregate light scattering properties by optimising simplified models to full light scattering calculations. It is found that there are no possible spherical models (at any size or refractive index) that well represent the light scattering in the visible or near-thermal infrared. As such, parameterisations of the light scattering as a function of the number of aggregate particles is presented as the most pragmatic choice for modelling distributions of black carbon when the large computational overheads of rigorous scattering calculations cannot be justified. This parameterisation can be analytically integrated to provide light scattering properties for lognormal distributions of black carbon fractal aggregates and return extinction cross sections with 0.1% accuracy for typical black carbon size distributions. Scattering cross sections and the asymmetry parameter can be obtained to within 3%.
机译:黑色碳分形聚集体具有复杂的形状,使得它们的光学性质的计算特别昂贵。这里,提出一种方法以通过优化简化模型来估计分形聚集光散射特性以满光散射计算。结果发现,没有可能的球形模型(在任何尺寸或折射率下),其良好地代表可见或近热红外线中的光散射。这样,当由于严格散射计算的大型计算开销不能合理时,将作为聚集粒子数量的函数的光散射的参数呈现为最务实的选择。可以分析地集成该参数化以提供黑色碳分形聚集体的伐木分布的光散射性能,并返回典型黑色碳尺寸分布的0.1%精度的消光横截面。可以获得散射横截面和不对称参数在3%以内。

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