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Enhanced Photocatalytic Degradation of Rhodamine B Using C/Fe Co-Doped Titanium Dioxide Coated on Activated Carbon

机译:使用C / Fe共掺杂二氧化物涂覆在活性炭上的C / Fe共掺杂二氧化钛增强光催化降解罗丹明B.

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Carbon and iron co-doped titanium dioxide catalyst coated on activated carbon (Fe-C-TiO2/AC) was successfully synthesized using the sol-gel method, followed by hydrothermal treatment. Commercial activated carbon was treated by HNO3 prior to being coated by the as-synthesized catalyst. The composite was characterized by XPS, XRD, UV-Vis spectrophotometry, IR, TEM, HR-TEM, and BET. The performance of the supported catalysts was evaluated in the degradation of rhodamine B (RhB) in the solution under visible-light irradiation. The results showed that, with the appropriate amount of activated carbon, prepared Fe-C-TiO2/AC catalysts exhibited higher catalytic activities and Fe-C-TiO2/AC system showed the best performance. The photocatalytic degradation efficiency of Fe-C-TiO2/AC was enhanced due to the synergistic effect between AC (adsorption effect) and Fe-C-TiO2 (photocatalysis effect). This facilitated the photocatalytic degradation of RhB by Fe-C-TiO2.
机译:使用溶胶 - 凝胶法成功地合成涂覆在活性炭(Fe-C-TiO2 / Ac)上的碳和铁共掺杂二氧化钛催化剂,然后通过水热处理合成。在由AS合成催化剂涂覆之前,通过HNO 3处理商业活性炭。复合材料的特征在于XPS,XRD,UV-Vis分光光度法,IR,TEM,HR-TEM和BET。在可见光照射下的溶液中罗丹明B(RHB)的降解中评价负载催化剂的性能。结果表明,通过适量的活性炭量,制备的Fe-C-TiO 2 / Ac催化剂表现出更高的催化活性,Fe-C-TiO2 / AC系统显示出最佳性能。由于AC(吸附效应)和Fe-C-TiO2(光催化效果)之间的协同效应,增强了Fe-C-TiO2 / Ac的光催化降解效率。这促进了Fe-C-TiO2的光催化降解了RHB。

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