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Elastic instabilities in planar elongational flow of monodisperse polymer solutions

机译:单分散聚合物溶液平面伸长流动的弹性稳定性

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We investigate purely elastic flow instabilities in the almost ideal planar stagnation point elongational flow field generated by a microfluidic optimized-shape cross-slot extensional rheometer (OSCER). We use time-resolved flow velocimetry and full-field birefringence microscopy to study the behavior of a series of well-characterized viscoelastic polymer solutions under conditions of low fluid inertia and over a wide range of imposed deformation rates. At low deformation rates the flow is steady and symmetric and appears Newtonian-like, while at high deformation rates we observe the onset of a flow asymmetry resembling the purely elastic instabilities reported in standard-shaped cross-slot devices. However, for intermediate rates, we observe a new type of elastic instability characterized by a lateral displacement and time-dependent motion of the stagnation point. At the onset of this new instability, we evaluate a well-known dimensionless criterion M that predicts the onset of elastic instabilities based on geometric and rheological scaling parameters. The criterion yields maximum values of M which compare well with critical values of M for the onset of elastic instabilities in viscometric torsional flows. We conclude that the same mechanism of tension acting along curved streamlines governs the onset of elastic instabilities in both extensional (irrotational) and torsional (rotational) viscoelastic flows.
机译:我们在微流体优化形状交叉槽延伸流变仪(OSCER)产生的几乎理想的平面停滞点伸长流场中调查纯粹的弹性流量。我们使用时间分辨的流量测速和全场双折射显微镜,以研究在低流体惯性条件下的一系列良好表征粘弹性聚合物溶液的行为,以及在各种施加的变形率。在低变形速率下,流量稳定且对称,类似于牛顿的速率,而在高变形速率下,我们观察了类似于标准形状交叉槽装置中报告的纯弹性不稳定性的流不对称的发作。然而,对于中间速率,我们观察到一种新型的弹性不稳定性,其特征在于横向位移和停滞点的时间依赖运动。在这种新的不稳定性的开始,我们评估了一个知名的无量纲标准M,其基于几何和流变缩放参数预测弹性稳定性的开始。该标准产生M的最大值,其与M的临界值相比,用于粘度扭转流动中的弹性稳定性的发作。我们得出结论,沿着弯曲的流线的相同张力作用机制治理延伸(无检测)和扭转(旋转)粘弹性流动中的弹性稳定性的发作。

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