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首页> 外文期刊>Fresenius environmental bulletin >FABRICATION OF SILVER-BASED VISIBLE-LIGHT-DRIVEN PHOTOCATALYST AND DEGRADATION OF ORGANIC POLLUTANTS IN WASTEWATER
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FABRICATION OF SILVER-BASED VISIBLE-LIGHT-DRIVEN PHOTOCATALYST AND DEGRADATION OF ORGANIC POLLUTANTS IN WASTEWATER

机译:银基可见光驱动的光催化剂的制备及废水中有机污染物的降解

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摘要

In recent years, photocatalysts focuses on narrow band gap semiconductors has attracted much attention in pollutants degradation due to its efficient degradation rate. Among the reported photocatalytic materials, Ag-based semiconductors as promising visible light-driven photocatalysts have aroused much interesting due to their strong visible light responsibility. In current work, a ternary plasmonic visible-light-driven photocatalyst Ag/Ag2W〇4/RGO (AAR) was successfully synthesized through a facile and effective hydrothermal method. The prepared AAR photocatalysts were characterized by X-ray diffraction pattern (XRD), Fourier transform infrared spectra (FT-IR), raman spectroscopy, field emission scanning clcctronmicroscopy (SEM) and ultra-violet-visible (UV-vis) diffuse reflectance speetTos-copy (DRS). It was found that (he AAR exhibited superior photocatalytic activity to bare Ag:W〇4 under visible light irradiation. The photocatalytic degradations of methylene blue (MB) dye pollutant over AAR photocatalyst were investigated. The significantly enhanced photocatalytic activity and stability of AAR photocatalyst could be attributed to the excellent clcctron-acccpting and transporting properties of reduced graphene oxide (RGO). The possible mechanism of photocatalytic activity enhancement was proposed.
机译:近年来,聚焦于窄带隙半导体的光催化剂由于其有效的降解速率而引起了污染物降解方面的广泛关注。在已报道的光催化材料中,基于银的半导体作为有前途的可见光驱动光催化剂,由于其对可见光的强烈反应而引起了人们的极大兴趣。在当前工作中,通过简便有效的水热方法成功地合成了三元等离激元可见光驱动的光催化剂Ag /Ag2W〇4/ RGO(AAR)。通过X射线衍射图谱(XRD),傅立叶变换红外光谱(FT-IR),拉曼光谱,场发射扫描电子显微镜(SEM)和紫外可见(UV-vis)漫反射比对表征的AAR光催化剂进行表征。复制(DRS)。结果表明:(他的AAR在可见光下对裸露的Ag:W〇4表现出优异的光催化活性。研究了亚甲基蓝(MB)染料污染物对AAR光催化剂的光催化降解。AAR光催化剂的光催化活性和稳定性显着增强归因于还原型氧化石墨烯(RGO)的优异的电子加速吸附和传输性能,提出了提高光催化活性的可能机理。

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