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机译:MINOS运动期间东地中海上空的气溶胶封闭和光散射系数的重建
The particulate mass (PM) concentration for fine aerosols at the MBL and FTsites averaged 17.4±4.7 µg/m3 and 11.2±3.2 µg/m3, respectively, and is among the highest reported in the literaturefor remote sites; more than 90% of this PM was composed equally ofammonium sulfate and carbonaceous aerosols. Comparison between the MBL andFT sites showed a slight vertical gradient for PM that was not observed fordust aerosols, which averaged 10.5±4.8 and 11.7±5.0 µg/m3 for the MBL and FT sites, respectively.
The results were used to reconstruct the ambient light scatteringcoefficient (σsp) that was measured at ambient RelativeHumidity (RH) for fine particles at the MBL site. Reconstruction of σsp was achieved using ratios of wet to dry scattering, f(RH), thatdepend on RH for ammonium sulfate, but are kept equal to 1 for POM. Thisresults in a low water adsorption for our organic-rich carbonaceousaerosols, although these aged biomass smoke aerosols are supposed to behighly oxidized. Mass scattering efficiencies of the main aerosol componentswere obtained by multivariate regression analysis, and were 2.66 and 4.19 m2/g(at the 95% confidence level) for dry ammonium sulfate and POM,respectively. The calculations indicate that one third of the reconstructedσsp was due to water uptake by ammonium sulfate aerosols,demonstrating their major role in the radiative aerosol properties in theeastern Mediterranean.
MBL和FT站点上的精细气溶胶的颗粒质量(PM)浓度平均为17.4±4.7 µg / m 3 sup>和11.2±3.2 µg / m 3 sup>,分别是文献中报道的偏远地区的最高值;超过90%的这种PM均由硫酸铵和碳质气溶胶组成。 MBL和FT站点之间的比较显示,PM的垂直梯度很小,而粉尘气溶胶则未观察到,MBL和FT站点的平均梯度分别为10.5±4.8和11.7±5.0 µg / m 3 sup>。 P style =“ line-height:20px;”>结果用于重建在环境相对湿度()下测量的环境光散射系数(σ sp i> sub>) RH i>)用于MBL处的细颗粒。 σ sp i> sub>的重建是通过干湿散射比 f i>( RH i>)实现的,该比率取决于< i> RH i>对于硫酸铵,但对于POM则保持等于1。尽管我们认为这些陈旧的生物质烟雾气溶胶被高度氧化,但是这导致我们富含有机物的碳质气溶胶的吸水率低。通过多元回归分析得出主要气溶胶组分的质量散射效率,干硫酸铵和POM分别为2.66和4.19 m 2 sup> / g(在95%置信度下)。计算表明,重建的σ sp i> sub>的三分之一是由于硫酸铵气雾剂吸收水,证明了它们在地中海东部辐射气雾剂特性中的主要作用。
机译:MINOS战役期间NO 3 sub>自由基在东地中海对流层氧化过程中的作用
机译:东地中海地区气溶胶的尺寸分离质量分布:季节变化和与AERONET柱状尺寸分布的比较
机译:MINOS运动期间的在线质谱气溶胶测量(克里特岛,2001年8月)
机译:用于实验室测试气溶胶和干燥环境气溶胶的测量和建模光散射系数之间的闭合
机译:开发并评估了用于HPLC的商用缩合成核光散射检测器原型以及用于与缩合成核光散射检测一起使用的电喷雾气溶胶的电晕放电中和器。
机译:时空变化和不同气溶胶类型对东地中海气溶胶光学深度的贡献
机译:MINOS运动期间东地中海上空的气溶胶物质封闭和光散射系数的重建
机译:地中海东部干旱环境冬末气溶胶特征与光散射的相互关系