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Causes of interannual variability over the southern hemispheric tropospheric ozone maximum

机译:南半球对流层臭氧最大值年际变化的原因

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摘要

We examine the relative contribution of processes controlling the interannual variability (IAV) of tropospheric ozone over four sub-regions of the southern hemispheric tropospheric ozone maximum (SHTOM) over a 20-year period. Our study is based on hindcast simulations from the National Aeronautics and Space Administration Global Modeling Initiative chemistry transport model (NASA GMI-CTM) of tropospheric and stratospheric chemistry, driven by assimilated Modern Era Retrospective Analysis for Research and Applications (MERRA) meteorological fields. Our analysis shows that over SHTOM region, the IAV of the stratospheric contribution is the most important factor driving the IAV of upper tropospheric ozone (270?hPa), where ozone has a strong radiative effect. Over the South Atlantic region, the contribution from surface emissions to the IAV of ozone exceeds that from stratospheric input at and below 430?hPa. Over the South Indian Ocean, the IAV of stratospheric ozone makes the largest contribution to the IAV of ozone with little or no influence from surface emissions at 270 and 430?hPa in austral winter. Over the tropical South Atlantic region, the contribution from IAV of stratospheric input dominates in austral winter at 270?hPa and drops to less than half but is still significant at 430?hPa. Emission contributions are not significant at these two levels. The IAV of lightning over this region also contributes to the IAV of ozone in September and December. Over the tropical southeastern Pacific, the contribution of the IAV of stratospheric input is significant at 270 and 430?hPa in austral winter, and emissions have little influence.
机译:我们研究了控制南半球对流层臭氧最大值(SHTOM)在20年期间的四个子区域中对流层臭氧年际变化(IAV)的过程的相对贡献。我们的研究基于对流层和平流层化学的美国国家航空航天局全球建模倡议化学模型(NASA GMI-CTM)的后验模拟,该模拟是由研究和应用的现代时代回顾性分析(MERRA)气象学领域驱动的。我们的分析表明,在SHTOM区域,平流层贡献的IAV是驱动对流层上层臭氧(270?hPa)IAV的最重要因素,其中臭氧具有很强的辐射作用。在南大西洋区域,地表排放对臭氧IAV的贡献超过了平流层输入(在430?hPa以下)的贡献。在南印度洋,平流层臭氧的IAV对臭氧的IAV贡献最大,而在南方冬季,在270和430?hPa的地表排放影响很小或没有影响。在南大西洋热带地区,平流层输入的IAV贡献在南方冬季为270?hPa时占主导地位,降至不到一半,但在430?hPa时仍显着。排放贡献在这两个级别上并不重要。该地区闪电的IAV也有助于9月和12月的臭氧IAV。在东南太平洋热带地区,平流层输入的IAV在南方冬季为270和430?hPa时非常重要,而排放几乎没有影响。

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