A gold(I)-catalyzed intramolecular oxidation-cyclopropanation sequence of 1,6-enynes: a convenient access to [n.1.0]bicycloalkanes

Deyun Qian; Junliang Zhang

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A gold(I)-catalyzed intramolecular oxidation-cyclopropanation sequence of 1,6-enynes: a convenient access to [n.1.0]bicycloalkanes

机译：金（I）催化的1,6-炔烃的分子内氧化-环丙烷化序列：方便地使用[n.1.0]双环烷烃

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摘要

A gold(I)-catalyzed tandem oxidation/cyclopropanation reaction of 1,6-enynes with an external oxidant has been developed. This quite simple and rapid strategy will provide a safe, mild and versatile avenue to numerous carbo- and hetero |n.1.0]bicyclic frameworks.

机译：已经开发了金（I）催化的1，6-炔烃与外部氧化剂的串联氧化/环丙烷化反应。这种非常简单，快速的策略将为众多的碳和杂双环[n.1.0]双环框架提供安全，温和且通用的途径。

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《Chemical Communications》 |2011年第39期|p.11152-11154|共3页
作者
Deyun Qian; Junliang Zhang;
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作者单位

Shanghai Key Laboratory of Green Chemistry and Chemical Processes, Department of Chemistry, East China Normal University,3663 N, Zhongshan Road, Shanghai 200062, P. R. China;

Shanghai Key Laboratory of Green Chemistry and Chemical Processes, Department of Chemistry, East China Normal University,3663 N, Zhongshan Road, Shanghai 200062, P. R. China,State key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences,P. R. China;

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2. Tetrahydrothiophene-Catalyzed Synthesis of Benzo[n.1.0] Bicycloalkanes [J] . Long-Wu Ye, Xiu-Li Sun, Chuan-Ying Li, The Journal of Organic Chemistry . 2007,第4期

机译：四氢噻吩催化合成苯并[n.1.0]双环烷烃
3. Palladium-Catalyzed Hydrohalogenation of 1,6-Enynes: Hydrogen Halide Salts and Alkyl Halides as Convenient HX Surrogates [J] . David A. Petrone, Ivan Franzoni, Juntao Ye, Journal of the American Chemical Society . 2017,第9期

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4. Gold Catalyzed 1,5- and 1,6-Propargylic Migrations of Ethers in Cycloisomerization of 1,6- and 1,7-Enynes. [C] . Cesar R. Solorio-Alvarado, Eloisa Jimenez-Nunez, Mihai Raducan European Symposium on Organic Chemistry . 2009

机译：黄金催化1,5-和1,6-丙基偏移的醚在1,6-和1,7-兴奋剂中的环旋异构化中。
5. Enantioselective palladium(II) catalyzed 1,6-enyne cyclizations: Methodology development and application to total synthesis [D] . Corkey, Britton Kenneth 2008

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6. Rhodium-Catalyzed Stereoselective Intramolecular 5 + 2 Cy-cloaddition of 3-Acyloxy-14-enyne and Alkene [O] . Xing-zhong Shu, Casi M. Schienebeck, Xiaoxun Li, -1

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机译：机械洞察Ru（ii） - 催化分子内正式3 + 2环加成（e）1,6-inynes

A gold(I)-catalyzed intramolecular oxidation-cyclopropanation sequence of 1,6-enynes: a convenient access to [n.1.0]bicycloalkanes

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