Carbonylation of the simplest persistent diaminocarbene

Tim Schulz; Christian Faerber; Michael Leibold; Clemens Bruhn; Wolfgang Baumann; Detlef Selent; Timo Porsch; Max C. Holthausen; Ulrich Siemeling

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Carbonylation of the simplest persistent diaminocarbene

机译：最简单的持久性二氨基卡宾的羰基化

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The reactions of the acyclic diaminocarbenes (Me_2N)_2C and (Ph_2N)-(iPr_2N)C with CO proceed in a 2:1 stoichiometric ratio, affording unprecedented betainic oxyallyl species of type [(R_2N)_2C]_2CO.

机译：无环二氨基卡宾（Me_2N）_2C和（Ph_2N）-（iPr_2N）C与CO的化学计量比为2：1，提供了前所未有的[（R_2N）_2C] _2CO类型的甜菜醛烯丙基。

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《Chemical Communications》 |2013年第61期|6834-6836|共3页
作者
Tim Schulz; Christian Faerber; Michael Leibold; Clemens Bruhn; Wolfgang Baumann; Detlef Selent; Timo Porsch; Max C. Holthausen; Ulrich Siemeling;
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Institute of Chemistry, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel, Germany;

Institute of Chemistry, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel, Germany;

Institute of Chemistry, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel, Germany;

Institute of Chemistry, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel, Germany;

Leibniz Institute for Catalysis e. V. at the University of Rostock, Albert-Einstein-Str. 29a, 18059 Rostock, Germany;

Leibniz Institute for Catalysis e. V. at the University of Rostock, Albert-Einstein-Str. 29a, 18059 Rostock, Germany;

Institut fuer Anorganische und Anafytische Chemie, Johann Wolfgang Goethe-Unnersitaet Frankfurt, Max-von-Laue-Str. 7, D-60438 Frankfurt am Main, Germany;

Institut fuer Anorganische und Anafytische Chemie, Johann Wolfgang Goethe-Unnersitaet Frankfurt, Max-von-Laue-Str. 7, D-60438 Frankfurt am Main, Germany;

Institute of Chemistry, University of Kassel, Heinrich-Plett-Str. 40, D-34132 Kassel, Germany;

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入库时间 2022-08-17 13:18:33

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1. Evaluation of benzthiazolidine-based formamidinium salts for the synthesis of penem-type β-lactams by uncatalysed carbonylation of acyclic diaminocarbenes [J] . MarkusJonek, HannesBuhl, MichaelLeibold, Zeitschrift fur Naturforschung, B. A Journal of Chemical Sciences . 2019,第4期

机译：基于苯并噻唑烷基甲脒盐的评价通过联胞菌二氨基甲苯的未储原甲基化合成PENEM型β-内酰胺
2. Diastereoselective synthesis of a bicyclic β-lactam with penicillin G-like spectrum of activity by carbonylation of an acyclic diaminocarbene [J] . Tim Schulz, Christian Faerber, Michael Leibold, Chemical Communications . 2014,第18期

机译：通过非环二氨基卡宾的羰基化非对映选择性合成具有青霉素G样活性的双环β-内酰胺
3. New Stable and Persistent Acyclic Diaminocarbenes [J] . Schulz Tim, Weismann Daniel, Wallbaum Lars, Chemistry: A European journal . 2015,第40期

机译：新型稳定持久的无环二氨基卡宾
4. Catalytic Activity of Acyclic Diaminocarbene (Derived from Formamidinium Salt)-Rhodium Complexes [C] . Daisuke Imao, Tetsuo Ohta, Yoshihiko Ito Symposium on Organometallic Chemistry . 2004

机译：无环二氨基甲苯（衍生自甲脒盐）催化活性 - HHODIUM络合物
5. Novel reactivity of silver isocyanide complexes and palladium bis(acyclic diaminocarbenes) as catalyst for the Nazarov cyclization [D] . Miranda, Anthea Jacinta 2009

机译：异氰酸银络合物和钯双（无环二氨基碳烯）作为纳扎罗夫环化催化剂的新型反应性
6. Acyclic diaminocarbene-based Thiele Chichibabin and Müller hydrocarbons [O] . Avijit Maiti, Shubhadeep Chandra, Biprajit Sarkar, 2020

机译：基于环纤维二氨基氨基酚素Chichibabin和Müller碳氢化合物
7. Cover Feature: Stable and Persistent Acyclic Diaminocarbenes with Cycloalkyl Substituents and Their Transformation to β-Lactams by Uncatalysed Carbonylation with CO (Chem. Eur. J. 6/2019) [O] . Lars Wallbaum, Daniel Weismann, Dennis Löber, 2019

机译：盖子特征：具有环烷基取代基的稳定和持续的无环二烷基苯，及其通过CO（Chem.Eur.J.6 / 2019）的非脱盐羰基化合物与β-内酰胺的转化。

Carbonylation of the simplest persistent diaminocarbene

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