Enhanced CO_2 sorption and selectivity by functionalization of a NbO-type metal-organic framework with polarized benzothiadiazole moieties

Chengling Song; Yabing He; Bin Li; Yajing Ling; Hailong Wang; Yunlong Feng; Rajamani Krishna; Banglin Chen

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Enhanced CO_2 sorption and selectivity by functionalization of a NbO-type metal-organic framework with polarized benzothiadiazole moieties

机译：通过极化的苯并噻二唑部分官能化的NbO型金属有机骨架提高了CO_2的吸附和选择性

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A new NbO-type metal-organic framework ZJNU-40 incorporating highly polarized benzothiadiazole moieties exhibits a high CO_2 uptake of 108 cm~3 g~(-1) at 296 K and 1 atm, as well as good adsorption selectivities of CO_2 over CH_4 and N_2 at room temperature, which is superior to that of the analogous MOF NOTT-101.

机译：结合了高极化苯并噻二唑部分的新型NbO型金属有机骨架ZJNU-40在296 K和1 atm时表现出108 cm〜3 g〜（-1）的高CO_2吸收率，以及对CH_4的良好CO_2吸附选择性。 N_2在室温下优于同类MOF NOTT-101。

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《Chemical Communications》 |2014年第81期|12105-12108|共4页
作者
Chengling Song; Yabing He; Bin Li; Yajing Ling; Hailong Wang; Yunlong Feng; Rajamani Krishna; Banglin Chen;
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College of Chemistry and Life Sciences, Zhejiang Normal University, Jinhua 321004, China;

College of Chemistry and Life Sciences, Zhejiang Normal University, Jinhua 321004, China;

Department of Chemistry, University of Texas at San Antonio, One UTSA Circle, San Antonio, Texas 78249-0698, USA;

College of Chemistry and Life Sciences, Zhejiang Normal University, Jinhua 321004, China;

Department of Chemistry, University of Texas at San Antonio, One UTSA Circle, San Antonio, Texas 78249-0698, USA;

College of Chemistry and Life Sciences, Zhejiang Normal University, Jinhua 321004, China;

Van't Hoff Institute for Molecular Sciences, University of Amsterdam Science Park 904, 1098 XH Amsterdam, The Netherlands;

Department of Chemistry, University of Texas at San Antonio, One UTSA Circle, San Antonio, Texas 78249-0698, USA;

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2. Significantly enhanced CO_2/CH_4 separation selectivity within a 3D prototype metal-organic framework functionalized with OH groups on pore surfaces at room temperature [J] . Chen Z., Xiang S., Arman H.D., European journal of inorganic chemistry . 2011,第14期

机译：在室温下用孔表面上的OH基官能化的3D原型金属有机框架内，CO_2 / CH_4分离选择性显着提高
3. High CO_2/N_2 and CO_2/CH_4 selectivity in a chiral metal-organic framework with contracted pores and multiple functionalities [J] . Xiaoxia Lv, Liangjun Li, Sifu Tang, Chemical Communications . 2014,第52期

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4. CO_2/N_2 adsorption selectivity using metal-organic framework MIL-101(Cr) for marine engine exhaust model [C] . V. J. Utami, Fayza Yulia, Nasruddin, International Tropical Renewable Energy Conference . 2020

机译：CO_2 / N_2使用金属 - 有机框架MIL-101（CR）用于海洋发动机排气模型的吸附选择性
5. Design, synthesis, characterization, and sorption properties of metal-organic frameworks and polyhedra based on [iron(3)oxide(R dioxide)(6)L(3)](0/+) clusters. [D] . Sudik, Andrea C. 2005

机译：设计，合成，表征，和基于[铁（3）氧化物（R二氧化）（6）L（3）]（0 / +）簇的多面体的吸附性能。
6. Framework-Flexibility Driven Selective Sorption of p-Xylene over Other Isomers by a Dynamic Metal-Organic Framework [O] . Soumya Mukherjee, Biplab Joarder, Biplab Manna, -1

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7. Enhanced CO2 sorption and selectivity by functionalization of a NbO-type metal-organic framework with polarized benzothiadiazole moieties [O] . Song, C., He, Y., Li, B., 2014

机译：通过极化的苯并噻二唑部分官能化的NbO型金属有机骨架提高了CO2的吸附和选择性

Enhanced CO_2 sorption and selectivity by functionalization of a NbO-type metal-organic framework with polarized benzothiadiazole moieties

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