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Influence of plasmonic resonant wavelength on energy transfer from an InCaN quantum well to quantum dots

机译:等离子体谐振波长对荷兰量子阱的能量转移对量子点的影响

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摘要

We demonstrated the enhanced nonradiative resonant energy transfer (NRET) process by localized surface plasmon (LSP) in the hybrid InGaN quantum well (QW) and CdSe/ZnS quantum dot (QD) structures. The LSP resonant wavelengths could be adjusted by silver (Ag) nanoparticle (NP) arrays annealed from different thicknesses of Ag films. The LSP resonant wavelengths that are close to the peak QD emission helped to enhance the NRET between the QW and QDs. Compared to the original NRET in the absence of Ag NPs, the LSP-enhanced NRET rate was improved by 6.9 times at the resonant wavelength of 600 nm. The calculated efficiency of the LSP-enhanced NRET was 73.1%, which was almost twice that of the original efficiency. Although Ag NPs exhibited a quenching effect, the LSP-enhanced NRET at the resonant wavelength of 465 nm enhanced QD luminescence, which demonstrated their potential use in energy conversion devices.
机译:我们证明了通过混合IngaN量子阱(QW)和CDSE / ZnS量子点(QD)结构中的局部表面等离子体(LSP)的增强的非接种共振能量转移(NRET)过程。 LSP共振波长可以通过来自不同厚度的Ag膜退火的银(Ag)纳米颗粒(NP)阵列进行调节。 接近峰值QD发射的LSP共振波长有助于增强QW和QD之间的数量。 与在没有Ag NPS的情况下的原始nRET相比,LSP增强的NRET速率在600nm的共振波长下提高了6.9倍。 LSP增强NRET的计算效率为73.1%,几乎是原始效率的两倍。 尽管Ag NPS表现出淬火效果,但LSP增强的NRET在465nm增强的QD发光中的共振波长,这证明了它们在能量转换装置中的潜在使用。

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  • 来源
    《Applied Physics Letters 》 |2021年第20期| 202103.1-202103.6| 共6页
  • 作者单位

    Advanced Photonics Center Southeast University Nanjing 210096 Jiangsu People's Republic of China;

    Advanced Photonics Center Southeast University Nanjing 210096 Jiangsu People's Republic of China;

    Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials School of Electronic Science and Engineering Nanjing University Nanjing 210093 People's Republic of China;

    Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials School of Electronic Science and Engineering Nanjing University Nanjing 210093 People's Republic of China;

    Advanced Photonics Center Southeast University Nanjing 210096 Jiangsu People's Republic of China;

    Advanced Photonics Center Southeast University Nanjing 210096 Jiangsu People's Republic of China;

    Advanced Photonics Center Southeast University Nanjing 210096 Jiangsu People's Republic of China;

    Advanced Photonics Center Southeast University Nanjing 210096 Jiangsu People's Republic of China;

    Advanced Photonics Center Southeast University Nanjing 210096 Jiangsu People's Republic of China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
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  • 正文语种 eng
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