Distribution characteristics of radionuclides in high-temperature melt phase during melt decontamination of decommissioned metal waste

摘要

The purpose of this paper is to investigate radionuiclides under various melting conditions that influence their distribution behavior during contaminated metal waste melting. Radioisotopes ~(60)Co, and ~(137)Cs were artificially used as the model contaminants. Most of the ~(60)Co remained in the ingot phase homogeneously and was barely present in the slag phase. The ~(137)Cs nuclides leave the melt caused by volatilization, and are essentially transferred to the slag and dust phase. They are then retained by filter systems. The captured ~(137)Cs in the slag phase is about 9% and 12% at a basicity of 0.82 and 1.42 respectively. The results of the demonstration test performed with a withdrawed steam generator from Young-Kwang Nuclear Power Plant shows that cobalt was distributed homogeneously on the ingot phase.