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Removal of strontium ions from simulated radioactive wastewater by vacuum membrane distillation

机译:真空膜蒸馏去除模拟放射性废水中的锶离子

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摘要

The removal of Sr2+ ions from simulated radioactive wastewater by vacuum membrane distillation (VMD) with hollow fiber membrane module was investigated. The removal efficiency of Sr2+ could maintain over 99.60%, and the membrane flux could maintain at 6.71 L.m(-2.)h(-1) when Sr2+ in the feed solution was about 10 mg/L. The effect of operating parameters on the membrane flux was examined, including feed temperature (30-70 degrees C), permeate side vacuum (0.10-0.98 atm) and feed flow velocity (10.5-41.8 L/h). Pressure buildup effect was observed during the process, which could interfere with the membrane flux. Pressure buildup effect was more serious when permeate side vacuum degree was over 0.9 atm. Considering energy consumption efficiency, the permeate side vacuum degree should be maintained at the turning point (0.9 atm) of the membrane flux. Dusty gas model could simulate the mass transfer of VMD process well with ARE (average relative error) of 5.31%. VMD is potential for the removal of Sr2+ ions from aqueous solution. (C) 2017 Elsevier Ltd. All rights reserved.
机译:研究了中空纤维膜组件通过真空膜蒸馏(VMD)去除模拟放射性废水中的Sr2 +离子。当进料溶液中的Sr2 +约为10 mg / L时,Sr2 +的去除效率可保持超过99.60%,膜通量可保持在6.71 L.m(-2。)h(-1)。检查了操作参数对膜通量的影响,包括进料温度(30-70摄氏度),渗透侧真空度(0.10-0.98 atm)和进料流速(10.5-41.8 L / h)。在此过程中观察到压力累积效应,这可能会干扰膜通量。当渗透侧真空度超过0.9 atm时,压力累积效果更为严重。考虑到能量消耗效率,渗透侧真空度应保持在膜通量的转折点(0.9个大气压)。 Dusty气体模型可以很好地模拟VMD过程的传质,其ARE(平均相对误差)为5.31%。 VMD具有从水溶液中去除Sr2 +离子的潜力。 (C)2017 Elsevier Ltd.保留所有权利。

著录项

  • 来源
    《Annals of nuclear energy》 |2017年第5期|363-368|共6页
  • 作者单位

    Tsinghua Univ, INET, Collaborat Innovat Ctr Adv Nucl Energy Technol, Beijing 100084, Peoples R China;

    Tsinghua Univ, INET, Collaborat Innovat Ctr Adv Nucl Energy Technol, Beijing 100084, Peoples R China|Tsinghua Univ, Beijing Key Lab Radioact Waste Treatment, Beijing 100084, Peoples R China;

    Tsinghua Univ, INET, Collaborat Innovat Ctr Adv Nucl Energy Technol, Beijing 100084, Peoples R China|Tsinghua Univ, Beijing Key Lab Radioact Waste Treatment, Beijing 100084, Peoples R China;

    Tsinghua Univ, INET, Collaborat Innovat Ctr Adv Nucl Energy Technol, Beijing 100084, Peoples R China;

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  • 正文语种 eng
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  • 关键词

    Vacuum membrane distillation; Hollow fiber membrane; Strontium; Radioactive wastewater; Dusty gas model;

    机译:真空膜蒸馏;中空纤维膜;锶;放射性废水;含尘气体模型;

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