Linear energy transfer of fission fragments of ~(235)U and nucleation of gas bubbles in aqueous solutions of uranyl nitrate

摘要

Fission fragments emitted in a fissile solution create tiny gas bubbles, the size of which is determined by the linear energy transfer (LET) of the particles. The LET of fission fragments of U-235 in aqueous solutions of uranyl nitrate has been determined, and using methods adapted from the literature, the size of gas bubbles generated along the tracks of these particles has been estimated, revealing important variations with respect to particle LET and solution properties. Empirical correlations are presented for the maximum radius of radiolytic gas bubbles in unsaturated solutions of uranyl nitrate as a function of solution temperature and concentration. These can be used to predict the critical concentration of dissolved hydrogen necessary for the appearance of gas voids during nuclear criticality transients. The findings are intended for use in a future model of nuclear criticality transients in aqueous fissile solutions for the purposes of nuclear criticality safety assessment. (C) 2020 Elsevier Ltd. All rights reserved.