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All-Dielectric Crescent Metasurface Sensor Driven by Bound States in the Continuum

机译:由绑定状态在连续体中驱动的全介电性新月形元件传感器

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摘要

Metasurfaces based on quasi-bound states in the continuum (quasi-BICs) constitute an emerging toolkit in nanophotonic sensing as they sustain high quality factor resonances and substantial near-field enhancements. It is demonstrated that silicon metasurfaces composed of crescent shaped meta-atoms provide tailored light-matter interaction controlled by the crescent geometry. Significantly, this metasurface not only exhibits a fundamental quasi-BIC resonance, but also supports a higher-order resonance with tunable electromagnetic field enhancement and advantageous properties for sensing. The higher-order resonance shows twice the sensitivity of the fundamental one for bulk refractive index sensing. It is further demonstrated that both the fundamental and higher-order resonances can be exploited for sensing ultrathin layers of biomolecules in air and buffer solutions. Specifically, when measuring in buffer solution, the figure of merit of the sensor, defined as the change in the spectral position of the resonance normalized to its full width at half maximum, is a factor of 2.5 larger for the higher-order resonance when compared to the fundamental one. Due to its high sensitivity and potential for straightforward microfluidic integration, the silicon crescent metasurface is ideally suited for real-time and in situ biosensing, enabling compact sensing devices for a wide range of diagnostic applications.
机译:基于连续体(准二语)的准界态的元锉构成了纳米光调节中的新兴工具包,因为它们维持了高质量因子共振和大量近场增强。据证明,由新月形元原子组成的硅质掩蚀提供由新月形几何体控制的定制的浅品相互作用。值得注意的是,这种质量表面不仅表现出基本的准二极管谐振,而且还支持具有可调谐电磁场增强和用于感测的有利特性的高阶谐振。高阶谐振显示了对散装折射率感测的基本敏感性的两倍。进一步证明,可以利用基本和高阶共振来检测空气和缓冲溶液中的超薄层的超薄层。具体地,当在缓冲溶液中测量时,传感器的优点图,定义为归一成向其全宽的共振的光谱位置的变化,比较时的高阶谐振的倍数为2.5倍。到基本的一个。由于其具有直接微流体集成的高灵敏度和潜力,因此硅新月形元表面非常适合实时和原位生物溶解,使得能够为各种诊断应用提供紧凑的传感设备。

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  • 来源
    《Advanced Functional Materials》 |2021年第46期|2104652.1-2104652.10|共10页
  • 作者单位

    Ludwig Maximilians Univ Munchen Fac Phys Nanoinst Munich Chair Hybrid Nanosyst D-80539 Munich Germany;

    Ludwig Maximilians Univ Munchen Fac Phys Nanoinst Munich Chair Hybrid Nanosyst D-80539 Munich Germany;

    Karlsruhe Inst Technol Inst Theoret Solid State Phys D-76131 Karlsruhe Germany;

    Karlsruhe Inst Technol Inst Theoret Solid State Phys D-76131 Karlsruhe Germany|Karlsruhe Inst Technol Inst Nanotechnol D-76021 Karlsruhe Germany;

    Ludwig Maximilians Univ Munchen Fac Phys Nanoinst Munich Chair Hybrid Nanosyst D-80539 Munich Germany|Imperial Coll London Dept Phys Blackett Lab London SW7 2AZ England;

    Ludwig Maximilians Univ Munchen Fac Phys Nanoinst Munich Chair Hybrid Nanosyst D-80539 Munich Germany;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    all-dielectric metasurfaces; biosensing; bound states in the continuum; optical label-free sensors; sensitivity;

    机译:全电介质元胶;生物传感;连续体中的绑定状态;无光标签传感器;灵敏度;

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