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The influence of past research on the design of experiments with dissolved organic matter and engineered nanoparticles

机译:过去的研究对溶解性有机物和工程纳米颗粒实验设计的影响

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摘要

To assess the environmental fate of engineered nanoparticles (ENPs), it is essential to understand their interactions with dissolved organic matter (DOM). The highly complex nature of the interactions between DOM and ENPs and other particulate matter (PM) requires investigating a wide range of material types under different conditions. However, despite repeated calls for an increased diversity of the DOM and PM studied, researchers increasingly focus on certain subsets of DOM and PM. Considering the discrepancy between the calls for more diversity and the research actually carried out, we hypothesize that materials that were studied more often are more visible in the scientific literature and therefore are more likely to be studied again. To investigate the plausibility of this hypothesis, we developed an agent-based model simulating the material choice in the experiments studying the interaction between DOM and PM between 1990 and 2015. The model reproduces the temporal trends in the choice of materials as well as the main properties of a network that displays the DOM and PM types investigated experimentally. The results, which support the hypothesis of a positive reinforcing material choice, help to explain why calls to increase the diversity of the materials studied are repeatedly made and why recent criticism states that the selection of materials is unbalanced.
机译:要评估工程纳米颗粒(ENP)的环境命运,必须了解它们与溶解有机物(DOM)的相互作用。 DOM与ENP和其他颗粒物(PM)之间相互作用的高度复杂性要求研究不同条件下的多种材料类型。然而,尽管一再呼吁增加所研究的DOM和PM的多样性,但研究人员越来越关注于DOM和PM的某些子集。考虑到对更多多样性的呼吁与实际进行的研究之间的差异,我们假设被研究更多的材料在科学文献中更为明显,因此更有可能再次被研究。为了研究该假设的合理性,我们在研究1990年至2015年间DOM和PM之间相互作用的实验中,开发了一种基于材料的模型来模拟材料的选择。该模型再现了材料选择的时间趋势以及主要显示DOM和PM类型的网络的实验性质。结果支持了积极的材料选择的假设,有助于解释为什么人们反复呼吁增加研究材料的多样性,以及为什么最近的批评指出材料的选择是不平衡的。

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