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The detection of carbon dioxide leaks using quasi-tomographic laser absorption spectroscopy measurements in variable wind

机译:在变风中使用准断层激光吸收光谱法测量二氧化碳泄漏

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摘要

Laser absorption spectroscopy (LAS) has been used over the last several decades for the measurement of trace gasses in the atmosphere. For over a decade, LAS measurements from multiple sources and tens of retroreflectors have been combined with sparse-sample tomography methods to estimate the 2-D distribution of trace gas concentrations and underlying fluxes from point-like sources. In this work, we consider the ability of such a system to detect and estimate the position and rate of a single point leak which may arise as a failure mode for carbon dioxide storage. The leak is assumed to be at a constant rate giving rise to a plume with a concentration and distribution that depend on the wind velocity. We demonstrate the ability of our approach to detect a leak using numerical simulation and also present a preliminary measurement.
机译:过去几十年来,激光吸收光谱法(LAS)已用于测量大气中的痕量气体。十多年来,来自多种来源和数十个回射器的LAS测量与稀疏样本层析成像方法相结合,以估算痕量气体浓度和来自点状来源的潜在通量的二维分布。在这项工作中,我们考虑了这种系统检测和估计单点泄漏的位置和速率的能力,该泄漏可能是二氧化碳存储的故障模式。假定泄漏的速率恒定,从而导致羽流的浓度和分布取决于风速。我们展示了我们的方法使用数值模拟检测泄漏的能力,并提出了初步的测量方法。

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