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Whispering-gallery nanocavity plasmon-enhanced Raman spectroscopy

机译:耳语画廊纳米腔等离子体激元拉曼光谱

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摘要

The synergy effect in nature could enable fantastic improvement of functional properties and associated effects. The detection performance of surface-enhanced Raman scattering (SERS) can be highly strengthened under the cooperation with other factors. Here, greatly-enhanced SERS detection is realized based on rolled-up tubular nano-resonators decorated with silver nanoparticles. The synergy effect between whispering-gallery-mode (WGM) and surface plasmon leads to an extra enhancement at the order of 105 compared to non-resonant flat SERS substrates, which can be well tuned by altering the diameter of micron- and nanotubes and the excitation laser wavelengths. Such synchronous and coherent coupling between plasmonics and photonics could lead to new principle and design for various sub-wavelength optical devices, e.g. plasmonic waveguides and hyperbolic metamaterials.
机译:自然界中的协同效应可以极大地改善功能特性和相关效应。在其他因素的共同作用下,可以大大增强表面增强拉曼散射(SERS)的检测性能。在此,基于装饰有银纳米颗粒的管状管状纳米谐振器实现了大大增强的SERS检测。与非共振平板SERS基板相比,耳语画廊模式(WGM)和表面等离子体激元之间的协同效应导致额外增强,幅度为10 5 。微米和纳米管的直径以及激发激光的波长。等离子体和光子之间的这种同步和相干耦合可能会导致各种亚波长光学器件(例如光子学)的新原理和设计。等离子体波导和双曲超材料。

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