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Superparamagnetic colloids in viscous fluids

机译:粘性流体中的超顺磁性胶体

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摘要

The influence of a magnetic field on the aggregation process of superparamagnetic colloids has been well known on short time for a few decades. However, the influence of important parameters, such as viscosity of the liquid, has received only little attention. Moreover, the equilibrium state reached after a long time is still challenging on some aspects. Indeed, recent experimental measurements show deviations from pure analytical models in extreme conditions. Furthermore, current simulations would require several years of computing time to reach equilibrium state under those conditions. In the present paper, we show how viscosity influences the characteristic time of the aggregation process, with experimental measurements in agreement with previous theories on transient behaviour. Afterwards, we performed numerical simulations on equivalent systems with lower viscosities. Below a critical value of viscosity, a transition to a new aggregation regime is observed and analysed. We noticed this result can be used to reduce the numerical simulation time from several orders of magnitude, without modifying the intrinsic physical behaviour of the particles. However, it also implies that, for high magnetic fields, granular gases could have a very different behaviour from colloidal liquids.
机译:几十年来,磁场对超顺磁性胶体聚集过程的影响是众所周知的。然而,诸如液体的粘度之类的重要参数的影响仅受到很少的关注。而且,长时间后达到的平衡状态在某些方面仍然具有挑战性。实际上,最近的实验测量表明,在极端条件下与纯分析模型存在偏差。此外,当前的仿真将需要几年的计算时间才能在这些条件下达到平衡状态。在本文中,我们通过实验测量与先前关于瞬态行为的理论相一致,展示了粘度如何影响聚集过程的特征时间。之后,我们在粘度较低的等效系统上进行了数值模拟。在粘度的临界值以下,观察到并分析了向新的聚集方式的转变。我们注意到该结果可用于将数值模拟时间从几个数量级减少,而无需修改粒子的固有物理行为。但是,这也暗示着,对于高磁场,粒状气体的行为可能与胶态液体非常不同。

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