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Tuning the motility and directionality of self-propelled colloids

机译:调整自推进胶体的运动性和方向性

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摘要

Microorganisms are able to overcome the thermal randomness of their surroundings by harvesting energy to navigate in viscous fluid environments. In a similar manner, synthetic colloidal microswimmers are capable of mimicking complex biolocomotion by means of simple self-propulsion mechanisms. Although experimentally the speed of active particles can be controlled by e.g. self-generated chemical and thermal gradients, an in-situ change of swimming direction remains a challenge. In this work, we study self-propulsion of half-coated spherical colloids in critical binary mixtures and show that the coupling of local body forces, induced by laser illumination, and the wetting properties of the colloid, can be used to finely tune both the colloid’s swimming speed and its directionality. We experimentally and numerically demonstrate that the direction of motion can be reversibly switched by means of the size and shape of the droplet(s) nucleated around the colloid, depending on the particle radius and the fluid’s ambient temperature. Moreover, the aforementioned features enable the possibility to realize both negative and positive phototaxis in light intensity gradients. Our results can be extended to other types of half-coated microswimmers, provided that both of their hemispheres are selectively made active but with distinct physical properties.
机译:微生物能够通过收集能量在粘性流体环境中导航来克服周围环境的热随机性。以类似的方式,合成的胶体微游泳器能够通过简单的自推进机制来模仿复杂的生物运动。尽管在实验上,活性颗粒的速度可以通过例如速度控制。自生化学梯度和热梯度,游泳方向的原位变化仍然是一个挑战。在这项工作中,我们研究了关键二元混合物中半包膜球形胶体的自推进作用,并显示了激光照射引起的局部体力的耦合以及胶体的润湿特性可用于微调两者。胶体的游泳速度及其方向性。我们通过实验和数值方法证明,可以通过围绕胶体成核的液滴的大小和形状来可逆地切换运动方向,具体取决于粒子半径和流体的环境温度。此外,前述特征使得有可能在光强度梯度中实现负和正趋光。我们的结果可以扩展到其他类型的半涂层微游泳器,只要它们的两个半球都被选择性激活,但具有不同的物理特性即可。

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