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Point-dipole approximation for small systems of strongly coupled radiating nanorods

机译:强耦合辐射纳米棒的小型系统的点偶极近似

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摘要

Systems of closely-spaced resonators can be strongly coupled by interactions mediated by scattered electromagnetic fields. In large systems the resulting response has been shown to be more sensitive to these collective interactions than to the detailed structure of individual resonators. Attempts to describe such systems have resulted in point-dipole approximations to resonators that are computationally efficient for large resonator ensembles. Here we provide a detailed study for the validity of point dipole approximations in small systems of strongly coupled plasmonic nanorods, including the cases of both super-radiant and subradiant excitations, where the characteristics of the excitation depends on the spatial separation between the nanorods. We show that over an appreciable range of rod lengths centered on 210 nm, when the relative separation kl in terms of the resonance wave number of light k satisfies klπ/2, the point electric dipole model becomes accurate. However, when the resonators are closer, the finite-size and geometry of the resonators modifies the excitation modes, in particular the cooperative mode line shifts of the point dipole approximation begin to rapidly diverge at small separations. We also construct simplified effective models by describing a pair of nanorods as a single effective metamolecule.
机译:间隔紧密的谐振器系统可以通过散射电磁场介导的相互作用而牢固地耦合在一起。在大型系统中,结果表明,对这些集体相互作用的响应比对单个谐振器的详细结构更敏感。试图描述这样的系统已经导致了对谐振器的点偶极近似,这对于大型谐振器集合在计算上是有效的。在这里,我们对强耦合等离子体纳米棒的小型系统中点偶极近似的有效性进行了详细研究,包括超辐射和亚辐射激发的情况,其中激发的特性取决于纳米棒之间的空间间隔。我们证明,在相对于光的共振波数k的相对间隔kl满足 k l π / 2 ,点电偶极子模型变得精确。然而,当谐振器更接近时,谐振器的有限尺寸和几何形状改变了激励模式,特别是点偶极子近似的协作模式线位移开始以很小的间隔迅速发散。我们还通过将一对纳米棒描述为单个有效的大分子来构建简化的有效模型。

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