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Omnidirectional broadband light absorption using large-area ultrathin lossy metallic film coatings

机译:使用大面积超薄有损金属膜涂层进行全向宽带光吸收

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摘要

Resonant absorbers based on nanostructured materials are promising for variety of applications including optical filters, thermophotovoltaics, thermal emitters, and hot-electron collection. One of the significant challenges for such microanoscale featured medium or surface, however, is costly lithographic processes for structural patterning which restricted from industrial production of complex designs. Here, we demonstrate lithography-free, broadband, polarization-independent optical absorbers based on a three-layer ultrathin film composed of subwavelength chromium (Cr) and oxide film coatings. We have measured almost perfect absorption as high as 99.5% across the entire visible regime and beyond (400–800 nm). In addition to near-ideal absorption, our absorbers exhibit omnidirectional independence for incidence angle over ±60 degrees. Broadband absorbers introduced in this study perform better than nanostructured plasmonic absorber counterparts in terms of bandwidth, polarization and angle independence. Improvements of such “blackbody” samples based on uniform thin-film coatings is attributed to extremely low quality factor of asymmetric highly-lossy Fabry-Perot cavities. Such broadband absorber designs are ultrathin compared to carbon nanotube based black materials, and does not require lithographic processes. This demonstration redirects the broadband super absorber design to extreme simplicity, higher performance and cost effective manufacturing convenience for practical industrial production.
机译:基于纳米结构材料的共振吸收器有望用于各种应用,包括滤光片,热光电,热发射器和热电子收集。然而,对于这种具有微米/纳米级特征的介质或表面的重大挑战之一是用于结构图案的昂贵的平版印刷工艺,其受限于复杂设计的工业生产。在这里,我们演示了基于三层超薄膜的无光刻,宽带,偏振无关的光吸收剂,该膜由亚波长铬(Cr)和氧化膜涂层组成。我们测得在整个可见光范围内(400-800 nm)甚至更高,几乎完美的吸收率高达99.5%。除了近乎理想的吸收,我们的吸收器还具有全方位的独立性,入射角超过±60度。在带宽,极化和角度独立性方面,本研究中介绍的宽带吸收器的性能优于纳米结构的等离子吸收器。这种基于均匀薄膜涂层的“黑体”样品的改进归因于非对称高损耗Fabry-Perot腔体的极低品质因数。与基于碳纳米管的黑色材料相比,这种宽带吸收器设计超薄,并且不需要光刻工艺。该演示将宽带超级吸收器设计重定向到极其简单,更高的性能和具有成本效益的制造便利性,以用于实际工业生产。

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