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Electric radiation mapping of silver/zinc oxide nanoantennas by using electron holography

机译:电子全息图绘制银/氧化锌纳米天线的电辐射图

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摘要

In this work, we report the fabrication of self-assembled zinc oxide nanorods grown on pentagonal faces of silver nanowires by using microwaves irradiation. The nanostructures resemble a hierarchal nanoantenna and were used to study the far and near field electrical metal-semiconductor behavior from the electrical radiation pattern resulting from the phase map reconstruction obtained using off-axis electron holography. As a comparison, we use electric numerical approximations methods for a finite number of ZnO nanorods on the Ag nanowires and show that the electric radiation intensities maps match closely the experimental results obtained with electron holography. The time evolution of the radiation pattern as generated from the nanostructure was recorded under in-situ radio frequency signal stimulation, in which the generated electrical source amplitude and frequency were varied from 0 to 5 V and from 1 to 10 MHz, respectively. The phase maps obtained from electron holography show the change in the distribution of the electric radiation pattern for individual nanoantennas. The mapping of this electrical behavior is of the utmost importance to gain a complete understanding for the metal-semiconductor (Ag/ZnO) heterojunction that will help to show the mechanism through which these receiving/transmitting structures behave at nanoscale level.
机译:在这项工作中,我们报告了使用微波辐射在银纳米线的五边形表面上生长的自组装氧化锌纳米棒的制造。纳米结构类似于层状纳米天线,并用于通过使用离轴电子全息图获得的相图重构从电辐射图研究远场和近场电金属-半导体行为。作为比较,我们对银纳米线上的有限数量的ZnO纳米棒使用了电数值近似方法,结果表明,电辐射强度图与电子全息图获得的实验结果非常吻合。在原位射频信号刺激下记录了由纳米结构产生的辐射图的时间演变,其中产生的电源幅度和频率分别从0到5 V和从1到10 MHz变化。从电子全息图获得的相位图显示了单个纳米天线的电辐射方向图分布的变化。为了完全了解金属-半导体(Ag / ZnO)异质结,该电学行为的映射至关重要,这将有助于显示这些接收/传输结构在纳米级的行为机理。

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