Impacts of meteorological parameters and emissions on decadal,interannual, and seasonal variations of atmospheric black carbon in the Tibetan Plateau

摘要

We quantified the impacts of variations in meteorological parameters and emissions on decadal, interannual, and seasonal variations of atmospheric black carbon (BC) in the Tibetan Plateau for 1980e2010 using a global 3-dimensional chemical transport model driven by the Modern Era Retrospective-analysis for Research and Applications (MERRA) meteorological fields. From 1980 to 2010, simulated surface BC concentrations and all-sky direct radiative forcing at the top of the atmosphere due to atmospheric BC increased by 0.15 mg mu00013 (63%) and by 0.23 W m 2 (62%), respectively, averaged over the Tibetan Plateau (75e105u0003E, 25e40u0003N). Simulated annual mean surface BC concentrations were in the range of 0.24e0.40 mg mu00013 averaged over the plateau for 1980e2010, with the decadal trends of 0.13 mg mu00013 per decade in the 1980s and 0.08 in the 2000s. The interannual variations were u00015.4% to 7.0% for deviation from the mean, 0.0062 mg mu00013 for mean absolute deviation, and 2.5% for absolute percent departure from the mean. Model sensitivity simulations indicated that the decadal trends of surface BC concentrations were mainly driven by changes in emissions, while the interannual variations were dependent on variations of both meteorological parameters and emissions. Meteorological parameters played a crucial role in driving the interannual variations of BC especially in the monsoon season.