Enhanced removal of benzene in nonthermal plasma with ozonation, flow recycling, and flow recirculation

摘要

A double stage AC/DC sequential high voltage reactor has been developed to study the decomposition of benzene in the air stream at atmospheric pressure. The removal efficiency was measured as a function of ozonation, flow recycling, and flow recirculation. Ozonation in the inlet, and recycling of the exhaust stream increased the removal of benzene, also with increasing of specific input energy(J l^-1) the effect of inlet flow ozonation on benzene decomposition was enhanced. The highest removal efficiency was obtained up to >99% in recirculation six times,while CO2 selectivity reached 99.9% and energy efficiency was 0.59 g kWh^-1. O3 production/decomposition > production of OH radicals > electronic and ionic collisions were indicated as the main mechanisms influencing benzene abatement in this research.