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Ultrafast structural dynamics studied by kilohertz time-resolved x-ray diffraction

机译:通过千赫兹时间分辨X射线衍射研究超快结构动力学

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摘要

Ultrashort multi-keV x-ray pulses are generated by electron plasma produced by the irradiation of femtosecond pulses on metals. These sub-picosecond x-ray pulses have extended the field of x-ray spectroscopy into the femtosecond time domain. However, pulse-to-pulse instability and long data acquisition time restrict the application of ultrashort x-ray systems operating at low repetition rates. Here we report on the performance of a femtosecond laser plasma-induced hard x-ray source that operates at 1-kHz repetition rate, and provides a flux of 2.0 × 1010 photons/s of Cu Kα radiation. Using this system for time-resolved x-ray diffraction experiments, we record in real time, the transient processes and structural changes induced by the interaction of 400-nm femtosecond pulse with the surface of a 200-nm thick Au (111) single crystal.
机译:飞秒脉冲在金属上产生的电子等离子体产生了超短的多keV x射线脉冲。这些亚皮秒级X射线脉冲将X射线光谱学的领域扩展到了飞秒时域。但是,脉冲间的不稳定性和较长的数据采集时间限制了以低重复频率运行的超短X射线系统的应用。在这里,我们报告了飞秒激光等离子体诱导的硬X射线源的性能,该硬X射线源以1 kHz的重复频率运行,并提供2.0×1010光子/ s的CuKα辐射通量。使用该系统进行时间分辨的X射线衍射实验,我们实时记录由400 nm飞秒脉冲与200 nm厚Au(111)单晶表面相互作用引起的瞬态过程和结构变化。

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