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NONSEQUENTIAL DOUBLE IONIZATION: A MINIMAL -CORRELATION APPROACH

机译:无序双电离:一种最小相关方法

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Nonsequential multiple ionization, where two or more electrons are ripped off the atom by the laser field in one coherent process, has attracted much interest for over a decade. Representative references include for experimental data and [7-16] for theoretical work; the not-too-recent work is covered in the review articles. Unlike above-threshold ionization (ATI) or higli-harmonic generation (HHG), this process cannot proceed in the absence of electron-electron correlation. Moreover, this correlation affords a sizeable premiu n for collaboration between the two electrons: for optimal laser intensities, the ratio of nonsequential over sequential double ionization, which materializes in the famous "knee", can be as high as six orders of magnitude. Until about a year ago, experimental data were restricted to the total yields. Recently, however, application of the COLTRIMS (cold-target recoil-ion-momentum spectroscopy) technique has allowed for the determination of the (three-dimensional) momenta of the ion and the electrons so that now the completely differential ionization rate has become accessible. Early on, rescattering was identified as a promising candidate for the physical mechanism of nonsequential double ionization (NSDI), the same mechanism that is known to be responsible for ATI and HHG. However, serious quantitative problems with this scenario precluded its acceptance until recently. This problem has now been revisited and appears to have been reso ved. More and more, rescattering is emerging as the dominant mechanism, but depending on the atomic species and the laser intensity, others may be required in addition. Thus far, there are only few theoretical results for the momentum distributions in NSDI and even fewer explicit calculations. The intense-field many-particle 5-matrix theory which has successfully reproduced many data for the total yields has been extended to calculations of the differential rates. A calcu-lationally simpler version of essentially the same model yields similar results in those parameter regimes where it is applicable. There is also a simulation on the basis of the time-dependent Schroedinger equation in one dimension for each electron. Much can be learned already from purely classical kinematical considerations along the lines of the so-called simple-man model of intense -laser atom processes. In this paper, we present a simple fully quantum-mechanical model hat is able to predict the momentum distributions for any given scenario, such as sequential ionization, nonsequential ionization via rescattering, or nonsequential ioniza-tion via rescattering into an excited state followed by tunneling. The absolute yield for a given scenario cannot be predicted, but its intensity dependence can. Most importantly, different scenarios generate very different momentum distributions. Comparison of the calculated with the measured momentum distributions then can support or discredit the respective scenario.
机译:在过去的十年中,不连续的多重电离引起了人们的极大兴趣,其中两个或多个电子在一个相干过程中被激光场从原子中剥离出来。代表性的参考文献包括实验数据和[7-16]的理论工作;评论文章涵盖了不太近期的工作。与阈值以上电离(ATI)或高谐波产生(HHG)不同,在没有电子与电子相关的情况下,无法进行此过程。而且,这种相关性为两个电子之间的协作提供了一个相当大的前提:对于最佳的激光强度,在著名的“膝盖”中实现的非顺序与顺序双电离的比率可以高达六个数量级。直到大约一年前,实验数据仅限于总产量。但是,最近,COLTRIMS(冷目标反冲离子动量能谱)技术的应用使得可以确定离子和电子的(三维)动量,因此现在可以使用完全差分电离率。早期,散射被认为是非顺序双电离(NSDI)物理机制的有前途的候选者,该机制与ATI和HHG已知的机制相同。但是,这种情况下严重的定量问题使它直到最近才被接受。现在已经重新考虑了这个问题,并且似乎已经解决了该问题。越来越多地将散射作为主要机理,但是取决于原子种类和激光强度,可能还需要其他散射。到目前为止,关于NSDI中动量分布的理论结果很少,甚至更少的显式计算。已经成功地复制了许多关于总产量的数据的强场多粒子5矩阵理论已经扩展到差分速率的计算。本质上相同的模型的计算简单版本在适用的那些参数方案中产生相似的结果。对于每个电子,在一维中还存在基于时间依赖性Schroedinger方程的模拟。从纯经典的运动学考虑,已经按照所谓的强激光原子过程的简单人模型学到了很多东西。在本文中,我们介绍了一种简单的完全量子力学模型,能够预测任何给定场景的动量分布,例如顺序电离,通过重散射进行非顺序电离,或通过重新散射为激发态然后隧穿进行非顺序电离。 。给定方案的绝对产量无法预测,但其强度依赖性可以预测。最重要的是,不同的场景会产生非常不同的动量分布。然后,将计算出的动量分布与测得的动量分布进行比较可以支持或抹杀相应的方案。

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