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Chemical weather forecast over the Yangtze River Delta region: Application of WRF-Chem

机译:长江三角洲地区的化学天气预报:WRF-CHEM的应用

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An operational system was built based on WRF-Chem model for the chemical weather forecast over the Yangtze River Delta (YRD) region. WRF-Chem is a fully coupled ‘online’ regional chemistry/transport model jointly developed by the National Center for Atmospheric Research (NCAR), National Oceanic and Atmospheric Administration (NOAA) etc. The model includes on-line calculations of dynamics, transport, dry and wet deposition, gas-phase and aerosol chemistry, radiation and photolysis, and surface emissions. The Streets emission inventory was implemented and fined in resolution by using TM (Thematic Mapper) land-use data. For the application, the model was updated by introducing the effect of aerosol on photolysis due to the high aerosol concentration over the YRD region. The operational system supplies regional distribution and station temporal variation products including O3, SO2, NOx (NO, NO2), CO, volatile organic compounds (VOCs) and aerosol (PM10, PM2.5, EC) etc. The observational data at five sites over Shanghai was used to evaluate the performance of the system. The results show that 1) the introduction of aerosol effect on photolysis distinctly increases ozone forecast, and 2) the numerical forecast has good performance in both concentration and temporal variability of ozone and aerosol, although it needs to be improved for very high concentration episodes. The operational system will greatly benefit the chemical weather forecast over the YRD region.
机译:根据长江三角洲(YRD)地区的化学天气预报为基础的运营系统。 WRF-Chem是一个完全耦合的‘在线’国家大气研究中心联合开发的区域化学/运输模式(NCAR),国家海洋和大气管理(NOAA)等。该模型包括在线计算动力学,运输,干燥和湿沉积,气相和气溶胶化学,辐射和光解,以及表面排放。通过使用TM(主题映射器)土地使用数据,在分辨率下实施和罚款街道排放库存。对于申请,由于YRD区域的高气溶胶浓度高,通过引入气溶胶对光解的效果来更新模型。操作系统提供区域分布和站时间变异产品,包括O3,SO2,NOx(NO,NO2),CO,挥发性有机化合物(VOC)和气溶胶(PM10,PM2.5,EC)等。五个地点的观察数据在上海,用于评估系统的表现。结果表明,1)引入气溶胶对光解的影响明显增加臭氧预测,而且2)数值预测在臭氧和气溶胶的浓度和时间变异性方面具有良好的性能,尽管需要改善非常高的浓度发作。运营系统将极大地利用YRD地区的化学天气预报。

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