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Generation and applications of attosecond pulses

机译:Attosecond脉冲的生成和应用

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The generation of ever shorter pulses is a key to exploring the dynamic behavior of matter on ever shorter time scales. Over the past decade novel ultrafast optical technologies have pushed the duration of laser pulses close to its natural limit, to the wave cycle, which lasts about one femtosecond (1 fs = 10{sup}-15 s) in the visible spectral range. Time-resolved measurements with these pulses are able to trace atomic motion in molecules and related chemical processes. However, electronic dynamics inside atoms often evolve on an attosecond (1 as = 10{sup}-18 s) timescale and require sub-femtosecond pulses for capturing them. This talk will review the recent generation, measurement and first applications of sub-femtosecond soft-X-ray pulses (near 100 eV). These X-ray pulses together with the few-cycle laser pulses used for their generation have opened the way to the development of a technique for attosecond sampling of electrons ejected from atoms. This is accomplished by probing electron emission with the oscillating electric field of the few-cycle laser pulse following an excitation of the atom by the synchronized sub-femtosecond X-ray pulse. Sampling the emission of photo electrons in this manner - with an apparatus that may be regarded as an optical-field-driven "streak camera" - allows time-resolved measurement of the X-ray pulse duration as well as of the laser field oscillations (fig. 1). Tracking the evolution of secondary (Auger) electron emission in addition to that of the primary (photo) electrons with the same system provides time-domain access to inner-shell atomic electron dynamics.
机译:较短的脉冲的产生是在更短的时间尺度上探索物质动态行为的关键。在过去的十年中,小说中的超快光学技术推动了靠近其自然极限的激光脉冲的持续时间,波动周期,该波循环持续在可见光谱范围内的一个飞秒(1 fs = 10 {sup} -15 s。与这些脉冲的时间分辨测量能够追踪分子中的原子运动和相关化学过程。然而,内部原子内的电子动力学通常在AttoSecond(1 AS = 10 {Sup} -18 S)时间尺度上,并且需要用于捕获它们的子模秒脉冲。此谈话将审查最近的生成,测量和第一次应用的子 - 飞秒软X射线脉冲(接近100eV)。这些X射线脉冲与其生成的几个循环激光脉冲一起开启了一种用于开发用于从原子喷射的电子的抗秒采样的技术的开发。这是通过通过同步的子飞秒X射线脉冲激励原子之后探测电子发射的电子发射来探测少循环激光脉冲的振荡电场。以这种方式对光电发射进行采样 - 具有可以被视为光场驱动的“条纹摄像机”的装置 - 允许时间分辨测量X射线脉冲持续时间以及激光场振荡(图。1)。除了具有相同系统的主要(照片)电子外,跟踪次级(螺旋钻)电子发射的演变提供了对内壳原子电子动力学的时域访问。

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