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BURN-UP CALIBRATION AND ERROR ANALYSIS OF HTR-10 SPHERICAL FUEL ELEMENTS BY GAMMA SPECTROSCOPY

机译:伽马能谱对HTR-10球形燃料元素的燃烧校准和误差分析

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The HTR-10 is a pebble bed High-temperature gas-cooled reactor (HTGR) with a nominal thermal power of 10 MW. The on-line nondestructive burn-up (BU) measurement for the spherical fuel elements with TRISO coated fuel particles is an important issue in the fuel management of the HTR-10. The HTR-10 employs an HPGe gamma spectroscopy system to determine the BU values of the discharged fuel elements, and the accuracy of the BU measurement system is a crucial issue. The calibration requirement and the absolute calibration method are discussed and analyzed in this paper. In this work, the long-lived fission product (137)~Cs is demonstrated as the best BU indicator in the HTR-10, whereas the inner-calibrating source method using the ratio of the amounts of (134)~Cs to (137)~Cs is not suitable. The BU value of a fuel element is proportional to the intensity of (137)~Cs gamma-ray and independent on the irradiation history of the fuel element, except for a small correction term related to the radioactive decay of (137)~Cs. The efficiency of the measurement system is calibrated by using a (137)~Cs standard source embedded into the center of a graphite sphere with the same size and the same graphite material as the fuel element, which was located at the measurement position of the fuel sphere, to eliminate the possible systematic errors from the measurement system. The difference in geometry and self-absorption between the BU measurement and the calibration measurement is corrected by applying the MCNP simulation. The error sources of the calibration results are analyzed, in which the uncertainty of the source activity (~5%) is found to dominate. The other major error sources include the fluctuation of the uranium loading in the fuel elements, the errors of the nuclear data, the counting errors of the detector, and thecorrection procedure for the detection efficiency. More than 1,900 fuel elements discharged from the HTR-10 have been measured by far, and the BU values of these elements spread in the range from 8.4±0.5 GWD/t to 20±1.0 GWD/t, where the relative errors of the burn-ups consist of the calibration errors about 5.2% and the counting errors around the order of 1%. The behavior of the measured burn-ups has been discussed qualitatively.
机译:HTR-10是一个卵石床高温气冷堆(HTGR),标称热功率为10 MW。具有TRISO涂层的燃料颗粒的球形燃料元件的在线无损燃烧(BU)测量是HTR-10燃料管理中的重要问题。 HTR-10采用HPGe伽马能谱系统确定排放的燃料元件的BU值,而BU测量系统的准确性是至关重要的问题。本文对标定要求和绝对标定方法进行了讨论和分析。在这项工作中,长寿命裂变产物(137)〜Cs被证明是HTR-10中最好的BU指示剂,而内标定源方法使用的是(134)〜Cs与(137)的数量之比。 )〜Cs不适合。燃料元件的BU值与(137)〜Csγ射线的强度成正比,并且与燃料元件的辐照历史无关,除了与(137)〜Cs的放射性衰变有关的小的校正项。测量系统的效率是通过使用(137)〜Cs标准源校准的,该标准源嵌入到位于燃料测量位置的与燃料元件相同尺寸和石墨材料的石墨球体中心。球,以消除测量系统中可能出现的系统误差。 BU测量和校准测量之间的几何形状和自吸收之间的差异可通过应用MCNP模拟进行校正。分析了校准结果的误差源,其中发现了源活动的不确定性(〜5%)。其他主要误差源包括燃料元件中铀负载的波动,核数据的误差,探测器的计数误差以及探测效率的校正程序。到目前为止,已经测量了从HTR-10排放的1,900多种燃料元素,这些元素的BU值分布在8.4±0.5 GWD / t至20±1.0 GWD / t的范围内,其中燃烧的相对误差-ups由大约5.2%的校准误差和大约1%的计数误差组成。已定性地讨论了测得的燃耗的行为。

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