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The synthesis and fabrication of horizontally aligned single-walled carbon nanotubes suspended across wide trenches for infrared detecting application

机译:水平排列的单壁碳纳米管的合成与制备,该碳纳米管悬浮在宽沟槽上,用于红外检测

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摘要

Horizontally aligned single-walled carbon nanotubes (SWNTs) were directly grown across trenches produced on SiO2/Si substrate, forming suspended aligned SWNTs over the trenches, and were fabricated with simple methods for infrared (IR) detection application. The horizontally aligned SWNTs can grow across trenches as wide as 40 mu m. The detector based on such SWNTs shows sharp and remarkable responses to the ON/OFF state changes of the IR lamp and IR radiation with different frequencies. The resistance of the SWNTs decreases about 22.86% under IR radiation with power less than 4 mW. The detector photoresponse to IR radiation of 120 Hz at room temperature could be easily observed. The response time constant is only about 500 mu s, which is more than two orders of magnitude shorter than that of the reported devices based on SWNT films and SWNT-polymer composites. This was achieved due to the absence of intertube junctions in our horizontally aligned SWNTs which exist in SWNT bundles and films and may reduce the signal conduction speed and the IR photoresponse performance. Instead of the bolometric model, the interband transition model is suggested to be the dominating origin of the photoresponse of our SWNT-based detector configuration.
机译:将水平排列的单壁碳纳米管(SWNT)直接生长在SiO2 / Si基板上产生的沟槽上,在沟槽上形成悬浮的排列的SWNT,并使用简单的红外(IR)检测方法进行制造。水平排列的单壁碳纳米管可以跨越40微米宽的沟槽生长。基于这种SWNT的检测器对不同频率的IR灯和IR辐射的ON / OFF状态变化显示出鲜明而显着的响应。在功率小于4 mW的IR辐射下,SWNT的电阻降低了约22.86%。在室温下,可以轻松观察到检测器对120 Hz红外辐射的光响应。响应时间常数仅为约500μs,比报道的基于SWNT薄膜和SWNT聚合物复合材料的器件的响应时间常数短两个数量级。之所以能够实现这一目标,是因为在我们水平排列的单壁碳纳米管中不存在管间连接点,而单壁碳纳米管存在于单壁碳纳米管束和薄膜中,可能会降低信号传导速度和红外光响应性能。代替辐射热模型,建议将频带间过渡模型作为我们基于SWNT的检测器配置的光响应的主要来源。

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