It's in the Fine Print: Erasable Three‐Dimensional Laser‐Printed Micro‐ and Nanostructures

Gr?fe David; Walden Sarah L.; Blinco James; Wegener Martin; Blasco Eva; Barner‐Kowollik Christopher

摘要

Abstract >3D printing, on all scales, is currently a vibrant topic in scientific and industrial research as it has enormous potential to radically change manufacturing. Owing to the inherent nature of the manufacturing process, 3D printed structures may require additional material to structurally support complex features. Such support material must be removed after printing—sometimes termed subtractive manufacturing—without adversely affecting the remaining structure. An elegant solution is the use of photoresists containing labile bonds that allow for controlled cleavage with specific triggers. Herein, we explore state‐of‐the‐art cleavable photoresists for 3D direct laser writing, as well as their potential to combine additive and subtractive manufacturing in a hybrid technology. We discuss photoresist design, feature resolution, cleavage properties, and current limitations of selected examples. Furthermore, we share our perspective on possible labile bonds, and their corresponding cleavage trigger, which we believe will have a critical impact on future applications and expand the toolbox of available cleavable photoresists. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P> 3D打印，在所有秤上，目前在科学和工业研究中是一种充满活力的话题，因为它具有巨大的潜力来改变制造。由于制造过程的固有性质，3D印刷结构可能需要额外的材料来在结构上支持复杂的特征。在印刷后必须除去这种支撑材料 - 有时被称为减效制造 - 而不会产生不利影响剩余结构。优雅的解决方案是使用含有不稳定键的光致抗蚀剂，其允许具有特异性触发的控制裂解。这里，我们探索用于3D直接激光书写的最先进的可切割的光致抗蚀剂，以及它们在混合技术中结合添加剂和减法制造的潜力。我们讨论光致抗蚀剂设计，特征分辨率，切割属性以及所选实施例的当前限制。此外，我们在可能的不稳定债券上分享了我们的观点，以及他们相信的相应解理触发器对未来的应用程序产生严重影响，并扩展可用于可切割的光致抗蚀剂的工具箱。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第16期</span><b style="margin: 0 2px;">|</b><span>共11页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gr?fe David&option=202" target="_blank" rel="nofollow">Gr?fe David;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Walden Sarah L.&option=202" target="_blank" rel="nofollow">Walden Sarah L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Blinco James&option=202" target="_blank" rel="nofollow">Blinco James;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wegener Martin&option=202" target="_blank" rel="nofollow">Wegener Martin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Blasco Eva&option=202" target="_blank" rel="nofollow">Blasco Eva;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Barner‐Kowollik Christopher&option=202" target="_blank" rel="nofollow">Barner‐Kowollik Christopher;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Centre for Materials Science School of Chemistry and PhysicsQueensland University of Technology (QUT)2 George Street QLD 4000 Brisbane Australia;</p> <p>Centre for Materials Science School of Chemistry and PhysicsQueensland University of Technology (QUT)2 George Street QLD 4000 Brisbane Australia;</p> <p>Centre for Materials Science School of Chemistry and PhysicsQueensland University of Technology (QUT)2 George Street QLD 4000 Brisbane Australia;</p> <p>Institute of Applied Physics (APH)Karlsruhe Institute of Technology (KIT)Engesserstrasse 18 76131 Karlsruhe Germany;</p> <p>Macromolecular ArchitecturesKarlsruhe Institute of Technology (KIT)Engesserstrasse 18 76131 Karlsruhe Germany;</p> <p>Centre for Materials Science School of Chemistry and PhysicsQueensland University of Technology (QUT)2 George Street QLD 4000 Brisbane Australia;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=3D printing&option=203" rel="nofollow">3D printing;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=degradable materials&option=203" rel="nofollow">degradable materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=direct laser writing&option=203" rel="nofollow">direct laser writing;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=labile bonds&option=203" rel="nofollow">labile bonds;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photochemistry&option=203" rel="nofollow">photochemistry;</a> </p> <div class="translation"> 机译：3D打印;可降解材料;直接激光书写;不稳定的粘合;光化学; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div 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class="enjiyixqcontent" href="/patent-detail/06130419444250.html">METHOD FOR MANUFACTURING 3-DIMENSIONAL NANOSTRUCTURES BY IMPRINT LITHOGRAPHY AND 3-DIMENSIONAL NANOSTRUCTURES THEREBY</a> <b>[P]</b> . <span> 外国专利：  KR20130068668A </span> <span> . 2013-06-26</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：通过光刻和三维纳米结构制造三维纳米结构的方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130459747454.html">Printed form of variable dimensions - has laser-printed areas with lines, squares, etc. in required dimensions</a> <b>[P]</b> . <span> 外国专利：  FR2692522A1 </span> <span> . 1993-12-24</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：可变尺寸的印刷形式-具有要求尺寸的带有线条，正方形等的激光印刷区域 </span> </p> </li> </ul> </div> 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